Low thermal noise mirror coatings utilising titanium dioxide and germanium dioxide mixtures

Fuente: arXiv
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Autores principales: Fazio, M., Martin, I. W., Hill, P., Yaala, M. Ben, Chicoine, M., Clark, C., Demos, N., Fejer, M. M., Gibson, D., Gras, S., Hough, J., Markosyan, A., McGhee, G., Rowan, S., Smith, J., Schiettekatte, F., Tait, S., Vajente, G., Reid, S.
Formato: Preprint
Publicado: 2025
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author Fazio, M.
Martin, I. W.
Hill, P.
Yaala, M. Ben
Chicoine, M.
Clark, C.
Demos, N.
Fejer, M. M.
Gibson, D.
Gras, S.
Hough, J.
Markosyan, A.
McGhee, G.
Rowan, S.
Smith, J.
Schiettekatte, F.
Tait, S.
Vajente, G.
Reid, S.
author_facet Fazio, M.
Martin, I. W.
Hill, P.
Yaala, M. Ben
Chicoine, M.
Clark, C.
Demos, N.
Fejer, M. M.
Gibson, D.
Gras, S.
Hough, J.
Markosyan, A.
McGhee, G.
Rowan, S.
Smith, J.
Schiettekatte, F.
Tait, S.
Vajente, G.
Reid, S.
contents Upgrades to ground-based gravitational-wave observatories will require mirror coatings with reduced thermal noise, enabling improved detector sensitivity and extended astrophysical reach. Recent studies have shown that optical coatings utilising amorphous materials that exhibit a larger fraction of corner-sharing between adjacent structural units of metal-centered polyhedra are a promising route for reducing mechanical dissipation and thus thermal noise at room temperature. We report on multilayer optical coatings that are fabricated using germanium dioxide mixed with titanium dioxide (TiO$_2$:GeO$_2$) for the high index layers, and silicon dioxide (SiO$_2$) for the low index material. Single layers of TiO$_2$:GeO$_2$ are characterised to optimise the mixture proportion and based on that highly reflective multilayer stacks were deposited. Exceptional optical absorption at 1064 nm below 1 part-per-million (ppm) is observed in the multilayer stacks after heat treatment. The annealing process also induces the formation of blisters which leads to increased optical scattering. However, there is indication that blisters can be suppressed by decreasing the water partial pressure in the deposition chamber. Direct thermal noise measurements provide experimental verification of a significant 25\% reduction of thermal noise over the mirrors currently employed, which combined with sub-ppm levels of optical absorption show the potential of TiO$_2$:GeO$_2$ to improve the sensitivity of gravitational-wave observatories.
format Preprint
id arxiv_https___arxiv_org_abs_2502_07679
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Low thermal noise mirror coatings utilising titanium dioxide and germanium dioxide mixtures
Fazio, M.
Martin, I. W.
Hill, P.
Yaala, M. Ben
Chicoine, M.
Clark, C.
Demos, N.
Fejer, M. M.
Gibson, D.
Gras, S.
Hough, J.
Markosyan, A.
McGhee, G.
Rowan, S.
Smith, J.
Schiettekatte, F.
Tait, S.
Vajente, G.
Reid, S.
Instrumentation and Detectors
Materials Science
Optics
Upgrades to ground-based gravitational-wave observatories will require mirror coatings with reduced thermal noise, enabling improved detector sensitivity and extended astrophysical reach. Recent studies have shown that optical coatings utilising amorphous materials that exhibit a larger fraction of corner-sharing between adjacent structural units of metal-centered polyhedra are a promising route for reducing mechanical dissipation and thus thermal noise at room temperature. We report on multilayer optical coatings that are fabricated using germanium dioxide mixed with titanium dioxide (TiO$_2$:GeO$_2$) for the high index layers, and silicon dioxide (SiO$_2$) for the low index material. Single layers of TiO$_2$:GeO$_2$ are characterised to optimise the mixture proportion and based on that highly reflective multilayer stacks were deposited. Exceptional optical absorption at 1064 nm below 1 part-per-million (ppm) is observed in the multilayer stacks after heat treatment. The annealing process also induces the formation of blisters which leads to increased optical scattering. However, there is indication that blisters can be suppressed by decreasing the water partial pressure in the deposition chamber. Direct thermal noise measurements provide experimental verification of a significant 25\% reduction of thermal noise over the mirrors currently employed, which combined with sub-ppm levels of optical absorption show the potential of TiO$_2$:GeO$_2$ to improve the sensitivity of gravitational-wave observatories.
title Low thermal noise mirror coatings utilising titanium dioxide and germanium dioxide mixtures
topic Instrumentation and Detectors
Materials Science
Optics
url https://arxiv.org/abs/2502.07679