Engineering 2D Van der Waals Electrode via MBE Grown Weyl Semimetal 1T-WTe2 for Enhanced Photodetection in InSe

Fuente: arXiv
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Auteurs principaux: Khan, Biswajit, Kandar, Santanu, Khan, Taslim, Bhattacharya, Kritika, Chowdahury, Nahid, Ghosh, Suprovat, Kumar, Pawan, Singh, Rajendra, Das, Samaresh
Format: Preprint
Publié: 2025
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author Khan, Biswajit
Kandar, Santanu
Khan, Taslim
Bhattacharya, Kritika
Chowdahury, Nahid
Ghosh, Suprovat
Kumar, Pawan
Singh, Rajendra
Das, Samaresh
author_facet Khan, Biswajit
Kandar, Santanu
Khan, Taslim
Bhattacharya, Kritika
Chowdahury, Nahid
Ghosh, Suprovat
Kumar, Pawan
Singh, Rajendra
Das, Samaresh
contents Achieving low contact resistance in advanced quantum electronic devices remains a critical challenge. With the growing demand for faster and energy-efficient devices, 2D contact engineering offers a promising solution. Beyond graphene, 1T-WTe2 has attracted attention for its excellent electrical transport, quantum phenomena, and Weyl semimetallic properties. Here, we demonstrate the direct wafer-scale growth of 1T-WTe2 via molecular beam epitaxy (MBE) and its use as a 2D contact for layered materials such as InSe. The 1T WTe2/InSe interface exhibits a barrier height nearly half that of conventional metal contacts, and its contact resistance is reduced by a factor of 21, effectively suppressing Fermi level pinning and enabling efficient electron injection. InSe/1T WTe2 photodetectors show broad photoresponsivity (0.14 to 217.58 A/W) under NIR to DUV illumination with fast rise/fall times of 42/126 ms, compared to lower responsivity (0.000865 A/W to 3.64 A/W) and slower response (150/144 ms) for InSe/Ti Au devices. The 1T WTe2/InSe devices thus exhibit approximately 60 times higher responsivity and 4 times faster response than conventional metal contacts. These results establish MBE-grown 1T-WTe2 as an effective 2D electrode, enhancing photodetection performance while simplifying device architecture, making it a strong candidate for next generation nanoelectronic and optoelectronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2502_13261
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Engineering 2D Van der Waals Electrode via MBE Grown Weyl Semimetal 1T-WTe2 for Enhanced Photodetection in InSe
Khan, Biswajit
Kandar, Santanu
Khan, Taslim
Bhattacharya, Kritika
Chowdahury, Nahid
Ghosh, Suprovat
Kumar, Pawan
Singh, Rajendra
Das, Samaresh
Optics
Achieving low contact resistance in advanced quantum electronic devices remains a critical challenge. With the growing demand for faster and energy-efficient devices, 2D contact engineering offers a promising solution. Beyond graphene, 1T-WTe2 has attracted attention for its excellent electrical transport, quantum phenomena, and Weyl semimetallic properties. Here, we demonstrate the direct wafer-scale growth of 1T-WTe2 via molecular beam epitaxy (MBE) and its use as a 2D contact for layered materials such as InSe. The 1T WTe2/InSe interface exhibits a barrier height nearly half that of conventional metal contacts, and its contact resistance is reduced by a factor of 21, effectively suppressing Fermi level pinning and enabling efficient electron injection. InSe/1T WTe2 photodetectors show broad photoresponsivity (0.14 to 217.58 A/W) under NIR to DUV illumination with fast rise/fall times of 42/126 ms, compared to lower responsivity (0.000865 A/W to 3.64 A/W) and slower response (150/144 ms) for InSe/Ti Au devices. The 1T WTe2/InSe devices thus exhibit approximately 60 times higher responsivity and 4 times faster response than conventional metal contacts. These results establish MBE-grown 1T-WTe2 as an effective 2D electrode, enhancing photodetection performance while simplifying device architecture, making it a strong candidate for next generation nanoelectronic and optoelectronic devices.
title Engineering 2D Van der Waals Electrode via MBE Grown Weyl Semimetal 1T-WTe2 for Enhanced Photodetection in InSe
topic Optics
url https://arxiv.org/abs/2502.13261