Impact of Pressure and Apical Oxygen Vacancies on Superconductivity in La$_3$Ni$_2$O$_7$

Fuente: arXiv
Guardado en:
Detalles Bibliográficos
Autores principales: Lu, Chen, Zhang, Ming, Pan, Zhiming, Wu, Congjun, Yang, Fan
Formato: Preprint
Publicado: 2025
Materias:
Acceso en línea:
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
_version_ 1866909980474474496
author Lu, Chen
Zhang, Ming
Pan, Zhiming
Wu, Congjun
Yang, Fan
author_facet Lu, Chen
Zhang, Ming
Pan, Zhiming
Wu, Congjun
Yang, Fan
contents The bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure has recently emerged as a promising system for high-$T_c$ superconductivity. In this work, we investigate the fate of the superconducting properties in La$_3$Ni$_2$O$_{7}$ under pressure, focusing on the effects of structural deformation and apical oxygen vacancies. Employing a low-energy effective $t$-$J_{\parallel}$-$J_{\perp}$ model for the $3d_{x^2-y^2}$ orbitals within the slave-boson mean-field approach, we demonstrate that the pairing strength is significantly enhanced in the high-pressure tetragonal $I4/mmm$ phase compared to the ambient pressure orthorhombic $Amam$ phase. Furthermore, by simulating random configurations of apical oxygen vacancies, we show that oxygen vacancies suppress both pairing strength and superfluid density. These results underscore the critical role of pressure and oxygen stoichiometry in tuning the SC of La$_3$Ni$_2$O$_7$, providing key insights into optimizing its high-$T_c$ behavior.
format Preprint
id arxiv_https___arxiv_org_abs_2502_14324
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Impact of Pressure and Apical Oxygen Vacancies on Superconductivity in La$_3$Ni$_2$O$_7$
Lu, Chen
Zhang, Ming
Pan, Zhiming
Wu, Congjun
Yang, Fan
Superconductivity
Strongly Correlated Electrons
The bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure has recently emerged as a promising system for high-$T_c$ superconductivity. In this work, we investigate the fate of the superconducting properties in La$_3$Ni$_2$O$_{7}$ under pressure, focusing on the effects of structural deformation and apical oxygen vacancies. Employing a low-energy effective $t$-$J_{\parallel}$-$J_{\perp}$ model for the $3d_{x^2-y^2}$ orbitals within the slave-boson mean-field approach, we demonstrate that the pairing strength is significantly enhanced in the high-pressure tetragonal $I4/mmm$ phase compared to the ambient pressure orthorhombic $Amam$ phase. Furthermore, by simulating random configurations of apical oxygen vacancies, we show that oxygen vacancies suppress both pairing strength and superfluid density. These results underscore the critical role of pressure and oxygen stoichiometry in tuning the SC of La$_3$Ni$_2$O$_7$, providing key insights into optimizing its high-$T_c$ behavior.
title Impact of Pressure and Apical Oxygen Vacancies on Superconductivity in La$_3$Ni$_2$O$_7$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2502.14324