Quantum Emitters in Rhombohedral Boron Nitride

Fuente: arXiv
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Autori principali: Gale, Angus, Kianinia, Mehran, Horder, Jake, Tweedie, Connor, Singhal, Mridul, Scognamiglio, Dominic, Qi, Jiajie, Li, Kaihui, Verdi, Carla, Aharonovich, Igor, Toth, Milos
Natura: Preprint
Pubblicazione: 2025
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author Gale, Angus
Kianinia, Mehran
Horder, Jake
Tweedie, Connor
Singhal, Mridul
Scognamiglio, Dominic
Qi, Jiajie
Li, Kaihui
Verdi, Carla
Aharonovich, Igor
Toth, Milos
author_facet Gale, Angus
Kianinia, Mehran
Horder, Jake
Tweedie, Connor
Singhal, Mridul
Scognamiglio, Dominic
Qi, Jiajie
Li, Kaihui
Verdi, Carla
Aharonovich, Igor
Toth, Milos
contents Rhombohedral boron nitride (rBN) is an emerging wide-bandgap van der Waals (vdW) material that combines strong second-order nonlinear optical properties with the structural flexibility of layered 2D systems. Here we show that rBN hosts optically-addressable spin defects and single-photon emitters (SPEs). Both are fabricated deterministically, using site-specific techniques, and are compared to their analogues in hexagonal boron nitride (hBN). Emission spectra in hBN and rBN are compared, and computational models of defects in hBN and rBN are used to elucidate the debated atomic structure of the B-center SPE in BN. Our results establish rBN as a monolithic vdW platform that uniquely combines second-order nonlinear optical properties, optically addressable spin defects, and high-quality SPEs, opening new possibilities for integrated quantum and nonlinear photonics.
format Preprint
id arxiv_https___arxiv_org_abs_2502_15157
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Quantum Emitters in Rhombohedral Boron Nitride
Gale, Angus
Kianinia, Mehran
Horder, Jake
Tweedie, Connor
Singhal, Mridul
Scognamiglio, Dominic
Qi, Jiajie
Li, Kaihui
Verdi, Carla
Aharonovich, Igor
Toth, Milos
Optics
Materials Science
Rhombohedral boron nitride (rBN) is an emerging wide-bandgap van der Waals (vdW) material that combines strong second-order nonlinear optical properties with the structural flexibility of layered 2D systems. Here we show that rBN hosts optically-addressable spin defects and single-photon emitters (SPEs). Both are fabricated deterministically, using site-specific techniques, and are compared to their analogues in hexagonal boron nitride (hBN). Emission spectra in hBN and rBN are compared, and computational models of defects in hBN and rBN are used to elucidate the debated atomic structure of the B-center SPE in BN. Our results establish rBN as a monolithic vdW platform that uniquely combines second-order nonlinear optical properties, optically addressable spin defects, and high-quality SPEs, opening new possibilities for integrated quantum and nonlinear photonics.
title Quantum Emitters in Rhombohedral Boron Nitride
topic Optics
Materials Science
url https://arxiv.org/abs/2502.15157