Anisotropic Exchange Spin Model to Investigate the Curie Temperature Dispersion of Finite-Size L10-FePt Magnetic Nanoparticles

Fuente: arXiv
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Autori principali: Ochiai, Kohei, Tsuyama, Tomoyuki, Shimizu, Sumera, Zhang, Lei, Watanabe, Jin, Kudo, Fumito, Zhu, Jian-Gang, Okuno, Yoshishige
Natura: Preprint
Pubblicazione: 2025
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author Ochiai, Kohei
Tsuyama, Tomoyuki
Shimizu, Sumera
Zhang, Lei
Watanabe, Jin
Kudo, Fumito
Zhu, Jian-Gang
Okuno, Yoshishige
author_facet Ochiai, Kohei
Tsuyama, Tomoyuki
Shimizu, Sumera
Zhang, Lei
Watanabe, Jin
Kudo, Fumito
Zhu, Jian-Gang
Okuno, Yoshishige
contents We developed an anisotropic spin model that accounts for magnetic anisotropy and evaluated the Curie temperature (Tc) dispersion due to finite size effects in L10-FePt nanoparticles. In heat-assisted magnetic recording (HAMR) media, a next-generation magnetic recording technology, high-density recording is achieved by locally heating L10-FePt nanoparticles near their Tc and rapidly cooling them. However, variations in Tc caused by differences in particle size and shape can compromise recording stability and areal density capacity, making the control of Tc dispersion critical. In this study, we constructed atomistic LLG models to explicitly incorporate the spin exchange anisotropy of L10-FePt, based on parameters determined by first-principles calculations. Using this model, we evaluated the impact of particle size on Tc dispersion. As a result, (1) the Tc dispersion critical to the performance of HAMR can be reproduced, whereas it was previously underestimated by isotropic models and (2) approximately 70% of the experimentally observed Tc dispersion can be attributed to particle size effects. This research highlights the role of exchange anisotropy in amplifying finite-size effects and underscores the importance of size control in HAMR media.
format Preprint
id arxiv_https___arxiv_org_abs_2502_15247
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Anisotropic Exchange Spin Model to Investigate the Curie Temperature Dispersion of Finite-Size L10-FePt Magnetic Nanoparticles
Ochiai, Kohei
Tsuyama, Tomoyuki
Shimizu, Sumera
Zhang, Lei
Watanabe, Jin
Kudo, Fumito
Zhu, Jian-Gang
Okuno, Yoshishige
Materials Science
Mesoscale and Nanoscale Physics
We developed an anisotropic spin model that accounts for magnetic anisotropy and evaluated the Curie temperature (Tc) dispersion due to finite size effects in L10-FePt nanoparticles. In heat-assisted magnetic recording (HAMR) media, a next-generation magnetic recording technology, high-density recording is achieved by locally heating L10-FePt nanoparticles near their Tc and rapidly cooling them. However, variations in Tc caused by differences in particle size and shape can compromise recording stability and areal density capacity, making the control of Tc dispersion critical. In this study, we constructed atomistic LLG models to explicitly incorporate the spin exchange anisotropy of L10-FePt, based on parameters determined by first-principles calculations. Using this model, we evaluated the impact of particle size on Tc dispersion. As a result, (1) the Tc dispersion critical to the performance of HAMR can be reproduced, whereas it was previously underestimated by isotropic models and (2) approximately 70% of the experimentally observed Tc dispersion can be attributed to particle size effects. This research highlights the role of exchange anisotropy in amplifying finite-size effects and underscores the importance of size control in HAMR media.
title Anisotropic Exchange Spin Model to Investigate the Curie Temperature Dispersion of Finite-Size L10-FePt Magnetic Nanoparticles
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2502.15247