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Main Authors: Liu, Shuping, Ren, Miaomiao, Xiao, Wanting, Wang, Jun, Liu, Yuting, Serrano, Diana, Goldner, Philippe, Tang, Dingyuan, An, Xiantong, Wang, Fudong, Zhong, Manjin
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2502.16222
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author Liu, Shuping
Ren, Miaomiao
Xiao, Wanting
Wang, Jun
Liu, Yuting
Serrano, Diana
Goldner, Philippe
Tang, Dingyuan
An, Xiantong
Wang, Fudong
Zhong, Manjin
author_facet Liu, Shuping
Ren, Miaomiao
Xiao, Wanting
Wang, Jun
Liu, Yuting
Serrano, Diana
Goldner, Philippe
Tang, Dingyuan
An, Xiantong
Wang, Fudong
Zhong, Manjin
contents Rare earth ions (REI) in solid materials are among the leading systems for quantum technology applications. However, developing practical REI quantum devices with long-lived coherent states remains challenging due to great growth difficulties of high-quality REI materials and a lack of comprehensive understanding of REI's decoherence mechanisms. Here we realize a record optical coherence time of 421.5 $\pm$ 10.5 $μ$s for the $^7$F$_0\rightarrow^5$D$_0$ transition and more than 30 hours lifetime for the $^7$F$_0$ hyperfine spin states in Eu$^{3+}$:Y$_2$O$_3$ optical ceramics. We report the elimination of two-level-system induced optical decoherence in short-range ordered crystals. Meanwhile, a new decoherence mechanism caused by new kinds of perturbing magnetic centers is identified below 1.5 K. We further demonstrate the coherent light storage over 5 $μ$s by using the atomic frequency comb protocol. These results open up prospects for the realization of practical quantum memories and large scale quantum communications with REI optical ceramics.
format Preprint
id arxiv_https___arxiv_org_abs_2502_16222
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Ultralong-lived Coherent States in Eu$^{3+}$:Y$_2$O$_3$ Optical Ceramics for Quantum Memories
Liu, Shuping
Ren, Miaomiao
Xiao, Wanting
Wang, Jun
Liu, Yuting
Serrano, Diana
Goldner, Philippe
Tang, Dingyuan
An, Xiantong
Wang, Fudong
Zhong, Manjin
Quantum Physics
Rare earth ions (REI) in solid materials are among the leading systems for quantum technology applications. However, developing practical REI quantum devices with long-lived coherent states remains challenging due to great growth difficulties of high-quality REI materials and a lack of comprehensive understanding of REI's decoherence mechanisms. Here we realize a record optical coherence time of 421.5 $\pm$ 10.5 $μ$s for the $^7$F$_0\rightarrow^5$D$_0$ transition and more than 30 hours lifetime for the $^7$F$_0$ hyperfine spin states in Eu$^{3+}$:Y$_2$O$_3$ optical ceramics. We report the elimination of two-level-system induced optical decoherence in short-range ordered crystals. Meanwhile, a new decoherence mechanism caused by new kinds of perturbing magnetic centers is identified below 1.5 K. We further demonstrate the coherent light storage over 5 $μ$s by using the atomic frequency comb protocol. These results open up prospects for the realization of practical quantum memories and large scale quantum communications with REI optical ceramics.
title Ultralong-lived Coherent States in Eu$^{3+}$:Y$_2$O$_3$ Optical Ceramics for Quantum Memories
topic Quantum Physics
url https://arxiv.org/abs/2502.16222