Phase evolution of strong-field ionization

Fuente: arXiv
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Auteurs principaux: Hutcheson, Lynda R, Hartmann, Maximilian, Borisova, Gergana D, Birk, Paul, Hu, Shuyuan, Ott, Christian, Pfeifer, Thomas, van der Hart, Hugo W, Brown, Andrew C
Format: Preprint
Publié: 2025
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author Hutcheson, Lynda R
Hartmann, Maximilian
Borisova, Gergana D
Birk, Paul
Hu, Shuyuan
Ott, Christian
Pfeifer, Thomas
van der Hart, Hugo W
Brown, Andrew C
author_facet Hutcheson, Lynda R
Hartmann, Maximilian
Borisova, Gergana D
Birk, Paul
Hu, Shuyuan
Ott, Christian
Pfeifer, Thomas
van der Hart, Hugo W
Brown, Andrew C
contents We investigate the time-dependent evolution of the dipole phase shift induced by strong-field ionization (SFI) using attosecond transient absorption spectroscopy (ATAS) for time-delays where the pump-probe pulses overlap. We study measured and calculated time-dependent ATA spectra of the ionic 4d-5p transition in xenon, and present the time-dependent line shape parameters in the complex plane. We attribute the complex, attosecond-scale dynamics to the contribution of three distinct processes: accumulation of ionization, transient population, and reversible population of excited states arising from polarization of the ground state.
format Preprint
id arxiv_https___arxiv_org_abs_2502_19010
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Phase evolution of strong-field ionization
Hutcheson, Lynda R
Hartmann, Maximilian
Borisova, Gergana D
Birk, Paul
Hu, Shuyuan
Ott, Christian
Pfeifer, Thomas
van der Hart, Hugo W
Brown, Andrew C
Atomic Physics
We investigate the time-dependent evolution of the dipole phase shift induced by strong-field ionization (SFI) using attosecond transient absorption spectroscopy (ATAS) for time-delays where the pump-probe pulses overlap. We study measured and calculated time-dependent ATA spectra of the ionic 4d-5p transition in xenon, and present the time-dependent line shape parameters in the complex plane. We attribute the complex, attosecond-scale dynamics to the contribution of three distinct processes: accumulation of ionization, transient population, and reversible population of excited states arising from polarization of the ground state.
title Phase evolution of strong-field ionization
topic Atomic Physics
url https://arxiv.org/abs/2502.19010