Search for magnetic field expulsion in optically driven K$_3$C$_{60}$

Fuente: arXiv
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Auteurs principaux: De Vecchi, G., Buzzi, M., Jotzu, G., Fava, S., Gebert, T., Magnani, G., Pontiroli, D., Riccò, M., Cavalleri, A.
Format: Preprint
Publié: 2025
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author De Vecchi, G.
Buzzi, M.
Jotzu, G.
Fava, S.
Gebert, T.
Magnani, G.
Pontiroli, D.
Riccò, M.
Cavalleri, A.
author_facet De Vecchi, G.
Buzzi, M.
Jotzu, G.
Fava, S.
Gebert, T.
Magnani, G.
Pontiroli, D.
Riccò, M.
Cavalleri, A.
contents Photoexcited K$_3$C$_{60}$ displays several properties reminiscent of equilibrium superconductivity, including transient optical spectra, pressure dependence, and I-V characteristics. However, these observations do not decisively establish non-equilibrium superconductivity, which would be conclusively evidenced by transient Meissner diamagnetism, as shown recently in driven YBa$_2$Cu$_3$O$_{6.48}$. Here, we search for transient magnetic field expulsion in K$_3$C$_{60}$ by measuring Faraday rotation in a magneto-optic material placed in its vicinity. Unlike in the case of homogeneous, insulating YBa$_2$Cu$_3$O$_{6.48}$, inhomogeneous, metallic K$_3$C$_{60}$ powders reduce the size of the effect. With the $\sim50$ nT magnetic field resolution achieved in our experiments, we provide an upper limit for the photo-induced diamagnetic volume susceptibility ($χ_v>-0.1$). On this basis, we conclude that the photo-induced phase has weaker diamagnetism than superconducting K$_3$C$_{60}$ at zero temperature. Yet, from recent nonlinear transport measurements in this granular material, we expect a light-induced state similar to the equilibrium superconductor near 0.8 T$_c$, for which $χ_v>-0.1$. A definitive conclusion on the presence or absence of Meissner diamagnetism cannot be made for K$_3$C$_{60}$ with the current resolution.
format Preprint
id arxiv_https___arxiv_org_abs_2502_20276
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Search for magnetic field expulsion in optically driven K$_3$C$_{60}$
De Vecchi, G.
Buzzi, M.
Jotzu, G.
Fava, S.
Gebert, T.
Magnani, G.
Pontiroli, D.
Riccò, M.
Cavalleri, A.
Superconductivity
Strongly Correlated Electrons
Photoexcited K$_3$C$_{60}$ displays several properties reminiscent of equilibrium superconductivity, including transient optical spectra, pressure dependence, and I-V characteristics. However, these observations do not decisively establish non-equilibrium superconductivity, which would be conclusively evidenced by transient Meissner diamagnetism, as shown recently in driven YBa$_2$Cu$_3$O$_{6.48}$. Here, we search for transient magnetic field expulsion in K$_3$C$_{60}$ by measuring Faraday rotation in a magneto-optic material placed in its vicinity. Unlike in the case of homogeneous, insulating YBa$_2$Cu$_3$O$_{6.48}$, inhomogeneous, metallic K$_3$C$_{60}$ powders reduce the size of the effect. With the $\sim50$ nT magnetic field resolution achieved in our experiments, we provide an upper limit for the photo-induced diamagnetic volume susceptibility ($χ_v>-0.1$). On this basis, we conclude that the photo-induced phase has weaker diamagnetism than superconducting K$_3$C$_{60}$ at zero temperature. Yet, from recent nonlinear transport measurements in this granular material, we expect a light-induced state similar to the equilibrium superconductor near 0.8 T$_c$, for which $χ_v>-0.1$. A definitive conclusion on the presence or absence of Meissner diamagnetism cannot be made for K$_3$C$_{60}$ with the current resolution.
title Search for magnetic field expulsion in optically driven K$_3$C$_{60}$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2502.20276