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Main Authors: Koll, Lisa-Marie, Jensen, Simon Vendelbo Bylling, van Essen, Pieter J., de Keijzer, Brian, Olsson, Emilia, Cottom, Jon, Witting, Tobias, Husakou, Anton, Vrakking, Marc J. J., Madsen, Lars Bojer, Kraus, Peter M., Jürgens, Peter
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2502.20564
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author Koll, Lisa-Marie
Jensen, Simon Vendelbo Bylling
van Essen, Pieter J.
de Keijzer, Brian
Olsson, Emilia
Cottom, Jon
Witting, Tobias
Husakou, Anton
Vrakking, Marc J. J.
Madsen, Lars Bojer
Kraus, Peter M.
Jürgens, Peter
author_facet Koll, Lisa-Marie
Jensen, Simon Vendelbo Bylling
van Essen, Pieter J.
de Keijzer, Brian
Olsson, Emilia
Cottom, Jon
Witting, Tobias
Husakou, Anton
Vrakking, Marc J. J.
Madsen, Lars Bojer
Kraus, Peter M.
Jürgens, Peter
contents Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics within crystalline structures. In this study, we employed extreme ultraviolet (XUV) high-harmonic interferometry with phase-locked XUV pulse pairs to investigate excitation-induced bandgap dynamics in solids. Our experiments on amorphous SiO2 and crystalline MgO, complemented by analytical modeling and semiconductor Bloch equation simulations, reveal a correlation between transient bandgap modifications and variations in the phase of harmonic emission. These findings suggest a potential pathway for sub-cycle, all-optical control of band structure modifications, advancing prospects for petahertz-scale electronic applications and attosecond diagnostics of carrier dynamics.
format Preprint
id arxiv_https___arxiv_org_abs_2502_20564
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Extreme Ultraviolet High-Harmonic Interferometry of Excitation-Induced Bandgap Dynamics in Solids
Koll, Lisa-Marie
Jensen, Simon Vendelbo Bylling
van Essen, Pieter J.
de Keijzer, Brian
Olsson, Emilia
Cottom, Jon
Witting, Tobias
Husakou, Anton
Vrakking, Marc J. J.
Madsen, Lars Bojer
Kraus, Peter M.
Jürgens, Peter
Optics
Materials Science
Interferometry is a fundamental technique in physics, enabling precise measurements through the interference of waves. High-harmonic generation (HHG) in solids has emerged as a powerful method for probing ultrafast electronic dynamics within crystalline structures. In this study, we employed extreme ultraviolet (XUV) high-harmonic interferometry with phase-locked XUV pulse pairs to investigate excitation-induced bandgap dynamics in solids. Our experiments on amorphous SiO2 and crystalline MgO, complemented by analytical modeling and semiconductor Bloch equation simulations, reveal a correlation between transient bandgap modifications and variations in the phase of harmonic emission. These findings suggest a potential pathway for sub-cycle, all-optical control of band structure modifications, advancing prospects for petahertz-scale electronic applications and attosecond diagnostics of carrier dynamics.
title Extreme Ultraviolet High-Harmonic Interferometry of Excitation-Induced Bandgap Dynamics in Solids
topic Optics
Materials Science
url https://arxiv.org/abs/2502.20564