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Main Authors: Chen, Yue, Chen, Haoran, Shen, Xi, Chen, Weizhao, Liu, Yi, Wu, Yizheng, Yuan, Zhe
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2502.20617
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author Chen, Yue
Chen, Haoran
Shen, Xi
Chen, Weizhao
Liu, Yi
Wu, Yizheng
Yuan, Zhe
author_facet Chen, Yue
Chen, Haoran
Shen, Xi
Chen, Weizhao
Liu, Yi
Wu, Yizheng
Yuan, Zhe
contents Using first-principles electronic structure calculation, we demonstrate the spin dissipation process in bulk Fe by orbital excitations within the energy bands of pure spin character. The variation of orbitals in the intraband transitions provides an efficient channel to convert spin to orbital angular momentum with spin-orbit interaction. This mechanism dominates the Gilbert damping of Fe below room temperature. The theoretical prediction is confirmed by the ferromagnetic resonance experiment performed on single-crystal Fe(001) films. A significant thickness-dependent damping oscillation is found at low temperature induced by the quantum well states of the corresponding energy bands. Our findings not only explain the microscopic nature of the recently reported ultralow damping of Fe-based alloys, but also help for the understanding of the transport and dissipation process of orbital currents.
format Preprint
id arxiv_https___arxiv_org_abs_2502_20617
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Orbital-excitation-dominated magnetization dissipation and quantum oscillation of Gilbert damping in Fe films
Chen, Yue
Chen, Haoran
Shen, Xi
Chen, Weizhao
Liu, Yi
Wu, Yizheng
Yuan, Zhe
Mesoscale and Nanoscale Physics
Materials Science
Using first-principles electronic structure calculation, we demonstrate the spin dissipation process in bulk Fe by orbital excitations within the energy bands of pure spin character. The variation of orbitals in the intraband transitions provides an efficient channel to convert spin to orbital angular momentum with spin-orbit interaction. This mechanism dominates the Gilbert damping of Fe below room temperature. The theoretical prediction is confirmed by the ferromagnetic resonance experiment performed on single-crystal Fe(001) films. A significant thickness-dependent damping oscillation is found at low temperature induced by the quantum well states of the corresponding energy bands. Our findings not only explain the microscopic nature of the recently reported ultralow damping of Fe-based alloys, but also help for the understanding of the transport and dissipation process of orbital currents.
title Orbital-excitation-dominated magnetization dissipation and quantum oscillation of Gilbert damping in Fe films
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2502.20617