Symmetry-Broken Kondo Screening and Zero-Energy Mode in the Kagome Superconductor CsV3Sb5

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Hauptverfasser: Tu, Yubing, Zhang, Zongyuan, Lu, Wenjian, Han, Tao, Lv, Run, Wang, Zhuying, Zhou, Zekun, Hou, Xinyuan, Hao, Ning, Wang, Zhenyu, Chen, Xianhui, Shan, Lei
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Veröffentlicht: 2025
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author Tu, Yubing
Zhang, Zongyuan
Lu, Wenjian
Han, Tao
Lv, Run
Wang, Zhuying
Zhou, Zekun
Hou, Xinyuan
Hao, Ning
Wang, Zhenyu
Chen, Xianhui
Shan, Lei
author_facet Tu, Yubing
Zhang, Zongyuan
Lu, Wenjian
Han, Tao
Lv, Run
Wang, Zhuying
Zhou, Zekun
Hou, Xinyuan
Hao, Ning
Wang, Zhenyu
Chen, Xianhui
Shan, Lei
contents The quantum states of matter reorganize themselves in response to defects, giving rise to emergent local excitations that imprint unique characteristics of the host states. While magnetic impurities are known to generate Kondo screening in a Fermi liquid and Yu-Shiba-Rusinov (YSR) states in a conventional superconductor, it remains unclear whether they can evoke distinct phenomena in the kagome superconductor AV3Sb5 (where A is K, Rb or Cs), which may host an orbital-antiferromagnetic charge density wave (CDW) state and an unconventional superconducting state driven by the convergence of topology, geometric frustration and electron correlations. In this work, we visualize the local density of states induced near various types of impurities in both the CDW and superconducting phases of CsV3-xMxSb5 (M = Ta, Cr) using scanning tunneling microscopy. We observe Kondo resonance states near magnetic Cr dopants. Notably, unlike in any known metal or CDW compound, the spatial pattern of Kondo screening breaks all in-plane mirror symmetries of the kagome lattice, suggesting an electronic chirality due to putative orbital loop currents. While Cooper pairs show relative insensitivity to nonmagnetic impurities, native V vacancies with weak magnetic moments induce a pronounced zero-bias conductance peak (ZBCP). This ZBCP coexists with trivial YSR states within the superconducting gap and does not split in energy with increasing tunneling transmission, tending instead to saturate. This behavior is reminiscent of signature of Majorana zero modes, which could be trapped by a sign-change boundary in the superconducting order parameter near a V vacancy, consistent with a surface topological superconducting state. Our findings provide a new approach to exploring novel quantum states on kagome lattices.
format Preprint
id arxiv_https___arxiv_org_abs_2502_20733
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Symmetry-Broken Kondo Screening and Zero-Energy Mode in the Kagome Superconductor CsV3Sb5
Tu, Yubing
Zhang, Zongyuan
Lu, Wenjian
Han, Tao
Lv, Run
Wang, Zhuying
Zhou, Zekun
Hou, Xinyuan
Hao, Ning
Wang, Zhenyu
Chen, Xianhui
Shan, Lei
Superconductivity
Strongly Correlated Electrons
The quantum states of matter reorganize themselves in response to defects, giving rise to emergent local excitations that imprint unique characteristics of the host states. While magnetic impurities are known to generate Kondo screening in a Fermi liquid and Yu-Shiba-Rusinov (YSR) states in a conventional superconductor, it remains unclear whether they can evoke distinct phenomena in the kagome superconductor AV3Sb5 (where A is K, Rb or Cs), which may host an orbital-antiferromagnetic charge density wave (CDW) state and an unconventional superconducting state driven by the convergence of topology, geometric frustration and electron correlations. In this work, we visualize the local density of states induced near various types of impurities in both the CDW and superconducting phases of CsV3-xMxSb5 (M = Ta, Cr) using scanning tunneling microscopy. We observe Kondo resonance states near magnetic Cr dopants. Notably, unlike in any known metal or CDW compound, the spatial pattern of Kondo screening breaks all in-plane mirror symmetries of the kagome lattice, suggesting an electronic chirality due to putative orbital loop currents. While Cooper pairs show relative insensitivity to nonmagnetic impurities, native V vacancies with weak magnetic moments induce a pronounced zero-bias conductance peak (ZBCP). This ZBCP coexists with trivial YSR states within the superconducting gap and does not split in energy with increasing tunneling transmission, tending instead to saturate. This behavior is reminiscent of signature of Majorana zero modes, which could be trapped by a sign-change boundary in the superconducting order parameter near a V vacancy, consistent with a surface topological superconducting state. Our findings provide a new approach to exploring novel quantum states on kagome lattices.
title Symmetry-Broken Kondo Screening and Zero-Energy Mode in the Kagome Superconductor CsV3Sb5
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2502.20733