Photon-drag photovoltaic effects and quantum geometric nature

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Hauptverfasser: Xie, Ying-Ming, Nagaosa, Naoto
Format: Preprint
Veröffentlicht: 2025
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author Xie, Ying-Ming
Nagaosa, Naoto
author_facet Xie, Ying-Ming
Nagaosa, Naoto
contents The bulk photovoltaic effect (BPVE) generates a direct current photocurrent under uniform irradiation and is a nonlinear optical effect traditionally studied in non-centrosymmetric materials. The two main origins of BPVE are the shift and injection currents, arising from transitions in electron position and electron velocity during optical excitation, respectively. Recently, it was proposed that photon-drag effects could unlock BPVE in centrosymmetric materials. However, experimental progress remains limited. In this work, we provide a comprehensive theoretical analysis of photon-drag effects inducing BPVE (photon-drag BPVE). Notably, we find that photon-drag BPVE can be directly linked to quantum geometric tensors. Additionally, we propose that photon-drag shift currents can be fully isolated from other current contributions in non-magnetic centrosymmetric materials. We apply our theory explicitly to the 2D topological insulator $1T'$-WTe$_2$. Furthermore, we investigate photon-drag BPVE in a centrosymmetric magnetic Weyl semimetal, where we demonstrate that linearly polarized light generates photon-drag shift currents.
format Preprint
id arxiv_https___arxiv_org_abs_2502_21002
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Photon-drag photovoltaic effects and quantum geometric nature
Xie, Ying-Ming
Nagaosa, Naoto
Mesoscale and Nanoscale Physics
Materials Science
Optics
The bulk photovoltaic effect (BPVE) generates a direct current photocurrent under uniform irradiation and is a nonlinear optical effect traditionally studied in non-centrosymmetric materials. The two main origins of BPVE are the shift and injection currents, arising from transitions in electron position and electron velocity during optical excitation, respectively. Recently, it was proposed that photon-drag effects could unlock BPVE in centrosymmetric materials. However, experimental progress remains limited. In this work, we provide a comprehensive theoretical analysis of photon-drag effects inducing BPVE (photon-drag BPVE). Notably, we find that photon-drag BPVE can be directly linked to quantum geometric tensors. Additionally, we propose that photon-drag shift currents can be fully isolated from other current contributions in non-magnetic centrosymmetric materials. We apply our theory explicitly to the 2D topological insulator $1T'$-WTe$_2$. Furthermore, we investigate photon-drag BPVE in a centrosymmetric magnetic Weyl semimetal, where we demonstrate that linearly polarized light generates photon-drag shift currents.
title Photon-drag photovoltaic effects and quantum geometric nature
topic Mesoscale and Nanoscale Physics
Materials Science
Optics
url https://arxiv.org/abs/2502.21002