Unambiguous determination of optical constants and thickness of ultrathin films by using optical anisotropic substrates

Fuente: arXiv
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Main Authors: Schaper, Sebastian, Duwe, Matthias, Wurstbauer, Ursula
Format: Preprint
Published: 2025
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author Schaper, Sebastian
Duwe, Matthias
Wurstbauer, Ursula
author_facet Schaper, Sebastian
Duwe, Matthias
Wurstbauer, Ursula
contents The unambiguous and universal determination of optical constants such as complex refractive indices (n, k) and thickness (d) in one measurement is typically confined for films with a thickness of more than 10~nm that hampers its application for ultra-thin films such as two-dimensional materials. We demonstrate that the commonly accepted limit of n, k, d coupling is overcome in ellipsometry by utilizing anisotropic substrates. In this way, ellipsometry allows to determine n, k and d simultaneously for thicknesses lower than 1~nm with high accuracy. Extensive simulations proof the potential of using anisotropic substrates for decoupling. The simultaneous determination of n, k and d is of great interest in several fields, two-dimensional materials, their heterostructures, ultra thin films for application in quantum technology, plasmonics and nano-photonics.
format Preprint
id arxiv_https___arxiv_org_abs_2502_21241
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Unambiguous determination of optical constants and thickness of ultrathin films by using optical anisotropic substrates
Schaper, Sebastian
Duwe, Matthias
Wurstbauer, Ursula
Optics
The unambiguous and universal determination of optical constants such as complex refractive indices (n, k) and thickness (d) in one measurement is typically confined for films with a thickness of more than 10~nm that hampers its application for ultra-thin films such as two-dimensional materials. We demonstrate that the commonly accepted limit of n, k, d coupling is overcome in ellipsometry by utilizing anisotropic substrates. In this way, ellipsometry allows to determine n, k and d simultaneously for thicknesses lower than 1~nm with high accuracy. Extensive simulations proof the potential of using anisotropic substrates for decoupling. The simultaneous determination of n, k and d is of great interest in several fields, two-dimensional materials, their heterostructures, ultra thin films for application in quantum technology, plasmonics and nano-photonics.
title Unambiguous determination of optical constants and thickness of ultrathin films by using optical anisotropic substrates
topic Optics
url https://arxiv.org/abs/2502.21241