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| Main Authors: | , , , , |
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| Format: | Preprint |
| Published: |
2025
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| Subjects: | |
| Online Access: | https://arxiv.org/abs/2503.00161 |
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| _version_ | 1866911518983979008 |
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| author | Cuenca, J. P. de Ara, T. Martinez-Garcia, A. Guzman, F. Sabater, C. |
| author_facet | Cuenca, J. P. de Ara, T. Martinez-Garcia, A. Guzman, F. Sabater, C. |
| contents | We present an in-depth study of electronic transport in atomic-sized gold contacts using Break-Junction (BJ) techniques under cryogenic and ambient conditions. Our experimental results, supported by classical molecular dynamics (CMD) simulations and ab initio calculations, provide compelling evidence for the formation of three-atom-thick structures in gold nanocontacts under tensile stress. These findings extend previous studies that confirmed the existence of one- and two-atom-thick chains. Beyond identifying these novel atomic configurations, we introduce a fast and robust calibration method for Break-Junction systems, leveraging the characteristic length of these structures to convert piezo displacement into absolute distance in angstroms. Our approach presents a novel and robust method for calibrating atomic distances in atomic conductor systems at both cryogenic and room temperatures. The results also enable the assessment of electrode sharpness, even at room conditions. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2503_00161 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Exploring Three-Atom-Thick Gold Structures as a Benchmark for Atomic-Scale Calibration of Break-Junction Systems Cuenca, J. P. de Ara, T. Martinez-Garcia, A. Guzman, F. Sabater, C. Mesoscale and Nanoscale Physics Materials Science We present an in-depth study of electronic transport in atomic-sized gold contacts using Break-Junction (BJ) techniques under cryogenic and ambient conditions. Our experimental results, supported by classical molecular dynamics (CMD) simulations and ab initio calculations, provide compelling evidence for the formation of three-atom-thick structures in gold nanocontacts under tensile stress. These findings extend previous studies that confirmed the existence of one- and two-atom-thick chains. Beyond identifying these novel atomic configurations, we introduce a fast and robust calibration method for Break-Junction systems, leveraging the characteristic length of these structures to convert piezo displacement into absolute distance in angstroms. Our approach presents a novel and robust method for calibrating atomic distances in atomic conductor systems at both cryogenic and room temperatures. The results also enable the assessment of electrode sharpness, even at room conditions. |
| title | Exploring Three-Atom-Thick Gold Structures as a Benchmark for Atomic-Scale Calibration of Break-Junction Systems |
| topic | Mesoscale and Nanoscale Physics Materials Science |
| url | https://arxiv.org/abs/2503.00161 |