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Main Authors: Wang, Hongteng, Li, Haichuan, Xin, Yijia, Chen, Weizhen, Liu, Haogen, Chen, Ying, Chen, Yaofei, Chen, Lei, Luo, Yunhan, Chen, Zhe, Liu, Gui-Shi
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2503.01549
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author Wang, Hongteng
Li, Haichuan
Xin, Yijia
Chen, Weizhen
Liu, Haogen
Chen, Ying
Chen, Yaofei
Chen, Lei
Luo, Yunhan
Chen, Zhe
Liu, Gui-Shi
author_facet Wang, Hongteng
Li, Haichuan
Xin, Yijia
Chen, Weizhen
Liu, Haogen
Chen, Ying
Chen, Yaofei
Chen, Lei
Luo, Yunhan
Chen, Zhe
Liu, Gui-Shi
contents As transparent electrodes, patterned silver nanowire (AgNW) networks suffer from noticeable pattern visibility, which is an unsettled issue for practical applications such as display. Here, we introduce a Gibbs-Thomson effect (GTE)-based patterning method to effectively reduce pattern visibility. Unlike conventional top-down and bottom-up strategies that rely on selective etching, removal, or deposition of AgNWs, our approach focuses on fragmenting nanowires primarily at the junctions through the GTE. This is realized by modifying AgNWs with a compound of diphenyliodonium nitrate and silver nitrate, which aggregates into nanoparticles at the junctions of AgNWs. These nanoparticles can boost the fragmentation of nanowires at the junctions under an ultralow temperature (75°C), allow pattern transfer through a photolithographic masking operation, and enhance plasmonic welding during UV exposure. The resultant patterned electrodes have trivial differences in transmittance (ΔT = 1.4%) and haze (ΔH = 0.3%) between conductive and insulative regions, with high-resolution patterning size down to 10 μm. To demonstrate the practicality of this novel method, we constructed a highly transparent, optoelectrical interactive tactile e-skin using the patterned AgNW electrodes.
format Preprint
id arxiv_https___arxiv_org_abs_2503_01549
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Patterning Silver Nanowire Network via the Gibbs-Thomson Effect
Wang, Hongteng
Li, Haichuan
Xin, Yijia
Chen, Weizhen
Liu, Haogen
Chen, Ying
Chen, Yaofei
Chen, Lei
Luo, Yunhan
Chen, Zhe
Liu, Gui-Shi
Systems and Control
As transparent electrodes, patterned silver nanowire (AgNW) networks suffer from noticeable pattern visibility, which is an unsettled issue for practical applications such as display. Here, we introduce a Gibbs-Thomson effect (GTE)-based patterning method to effectively reduce pattern visibility. Unlike conventional top-down and bottom-up strategies that rely on selective etching, removal, or deposition of AgNWs, our approach focuses on fragmenting nanowires primarily at the junctions through the GTE. This is realized by modifying AgNWs with a compound of diphenyliodonium nitrate and silver nitrate, which aggregates into nanoparticles at the junctions of AgNWs. These nanoparticles can boost the fragmentation of nanowires at the junctions under an ultralow temperature (75°C), allow pattern transfer through a photolithographic masking operation, and enhance plasmonic welding during UV exposure. The resultant patterned electrodes have trivial differences in transmittance (ΔT = 1.4%) and haze (ΔH = 0.3%) between conductive and insulative regions, with high-resolution patterning size down to 10 μm. To demonstrate the practicality of this novel method, we constructed a highly transparent, optoelectrical interactive tactile e-skin using the patterned AgNW electrodes.
title Patterning Silver Nanowire Network via the Gibbs-Thomson Effect
topic Systems and Control
url https://arxiv.org/abs/2503.01549