Ultrahigh free-electron Kerr nonlinearity in all-semiconductor waveguides for all-optical nonlinear modulation of mid-infrared light

Fuente: arXiv
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Autores principales: Álvarez-Pérez, Gonzalo, Hu, Huatian, Huang, Fangcheng, Otomalo, Tadele Orbula, Ortolani, Michele, Ciracì, Cristian
Formato: Preprint
Publicado: 2025
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author Álvarez-Pérez, Gonzalo
Hu, Huatian
Huang, Fangcheng
Otomalo, Tadele Orbula
Ortolani, Michele
Ciracì, Cristian
author_facet Álvarez-Pérez, Gonzalo
Hu, Huatian
Huang, Fangcheng
Otomalo, Tadele Orbula
Ortolani, Michele
Ciracì, Cristian
contents Nonlinear optical waveguides, particularly those harnessing the optical Kerr effect, are promising for advancing next-generation photonic technologies. Despite the Kerr effect`s ultrafast response, its inherently weak nonlinearity has hindered practical applications. Here, we explore free-electron-induced Kerr nonlinearities in all-semiconductor waveguides, revealing that longitudinal bulk plasmons (inherently nonlocal excitations) can generate exceptionally strong Kerr nonlinearities. We specifically develop a nonlinear eigenmode analysis integrated with semiclassical hydrodynamic theory to compute the linear and nonlinear optical responses originating from the quantum behavior of free electrons in heavily doped semiconductors. These waveguides achieve ultrahigh nonlinear coefficients exceeding 10$^7$ W$^{-1}$km$^{-1}$ and support long-propagating modes with propagation distances over 100 $μ$m. Additionally, we confirm the robustness of the nonlinear response under realistic conditions by considering viscoelastic and nonlinear damping mechanisms. Finally, we implement our all-semiconductor waveguides in a Mach-Zehnder interferometer, demonstrating efficient nonlinear modulation of the transmittance spectrum via the free-electron Kerr effect. This work evidences the transformative potential of free-electron nonlinearities in heavily doped semiconductors for photonic integrated circuits, paving the way for scalable on-chip nonlinear nanophotonic systems.
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institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Ultrahigh free-electron Kerr nonlinearity in all-semiconductor waveguides for all-optical nonlinear modulation of mid-infrared light
Álvarez-Pérez, Gonzalo
Hu, Huatian
Huang, Fangcheng
Otomalo, Tadele Orbula
Ortolani, Michele
Ciracì, Cristian
Optics
Quantum Physics
Nonlinear optical waveguides, particularly those harnessing the optical Kerr effect, are promising for advancing next-generation photonic technologies. Despite the Kerr effect`s ultrafast response, its inherently weak nonlinearity has hindered practical applications. Here, we explore free-electron-induced Kerr nonlinearities in all-semiconductor waveguides, revealing that longitudinal bulk plasmons (inherently nonlocal excitations) can generate exceptionally strong Kerr nonlinearities. We specifically develop a nonlinear eigenmode analysis integrated with semiclassical hydrodynamic theory to compute the linear and nonlinear optical responses originating from the quantum behavior of free electrons in heavily doped semiconductors. These waveguides achieve ultrahigh nonlinear coefficients exceeding 10$^7$ W$^{-1}$km$^{-1}$ and support long-propagating modes with propagation distances over 100 $μ$m. Additionally, we confirm the robustness of the nonlinear response under realistic conditions by considering viscoelastic and nonlinear damping mechanisms. Finally, we implement our all-semiconductor waveguides in a Mach-Zehnder interferometer, demonstrating efficient nonlinear modulation of the transmittance spectrum via the free-electron Kerr effect. This work evidences the transformative potential of free-electron nonlinearities in heavily doped semiconductors for photonic integrated circuits, paving the way for scalable on-chip nonlinear nanophotonic systems.
title Ultrahigh free-electron Kerr nonlinearity in all-semiconductor waveguides for all-optical nonlinear modulation of mid-infrared light
topic Optics
Quantum Physics
url https://arxiv.org/abs/2503.04711