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Main Authors: Chattoraj, Joyjit, Hamadicharef, Brahim, Chang, Teo Shi, Zeng, Yingzhi, Poh, Chee Kok, Chen, Luwei, Tan, Teck Leong
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2503.05607
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author Chattoraj, Joyjit
Hamadicharef, Brahim
Chang, Teo Shi
Zeng, Yingzhi
Poh, Chee Kok
Chen, Luwei
Tan, Teck Leong
author_facet Chattoraj, Joyjit
Hamadicharef, Brahim
Chang, Teo Shi
Zeng, Yingzhi
Poh, Chee Kok
Chen, Luwei
Tan, Teck Leong
contents While the Water-Gas Shift (WGS) reaction plays a crucial role in hydrogen production for fuel cells, finding suitable catalysts to achieve high yields for low-temperature WGS reactions remains a persistent challenge. Artificial Intelligence (AI) has shown promise in accelerating catalyst design by exploring vast candidate spaces, however, two key gaps limit its effectiveness. First, AI models primarily train on numerical data, which fail to capture essential text-based information, such as catalyst synthesis methods. Second, the cross-disciplinary nature of catalyst design requires seamless collaboration between AI, theory, experiments, and numerical simulations, often leading to communication barriers. To address these gaps, we present AceWGS, a Large Language Models (LLMs)-aided framework to streamline WGS catalyst design. AceWGS interacts with researchers through natural language, answering queries based on four features: (i) answering general queries, (ii) extracting information about the database comprising WGS-related journal articles, (iii) comprehending the context described in these articles, and (iv) identifying catalyst candidates using our proposed AI inverse model. We presented a practical case study demonstrating how AceWGS can accelerate the catalyst design process. AceWGS, built with open-source tools, offers an adjustable framework that researchers can readily adapt for a range of AI-accelerated catalyst design applications, supporting seamless integration across cross-disciplinary studies.
format Preprint
id arxiv_https___arxiv_org_abs_2503_05607
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle AceWGS: An LLM-Aided Framework to Accelerate Catalyst Design for Water-Gas Shift Reactions
Chattoraj, Joyjit
Hamadicharef, Brahim
Chang, Teo Shi
Zeng, Yingzhi
Poh, Chee Kok
Chen, Luwei
Tan, Teck Leong
Computation and Language
Artificial Intelligence
While the Water-Gas Shift (WGS) reaction plays a crucial role in hydrogen production for fuel cells, finding suitable catalysts to achieve high yields for low-temperature WGS reactions remains a persistent challenge. Artificial Intelligence (AI) has shown promise in accelerating catalyst design by exploring vast candidate spaces, however, two key gaps limit its effectiveness. First, AI models primarily train on numerical data, which fail to capture essential text-based information, such as catalyst synthesis methods. Second, the cross-disciplinary nature of catalyst design requires seamless collaboration between AI, theory, experiments, and numerical simulations, often leading to communication barriers. To address these gaps, we present AceWGS, a Large Language Models (LLMs)-aided framework to streamline WGS catalyst design. AceWGS interacts with researchers through natural language, answering queries based on four features: (i) answering general queries, (ii) extracting information about the database comprising WGS-related journal articles, (iii) comprehending the context described in these articles, and (iv) identifying catalyst candidates using our proposed AI inverse model. We presented a practical case study demonstrating how AceWGS can accelerate the catalyst design process. AceWGS, built with open-source tools, offers an adjustable framework that researchers can readily adapt for a range of AI-accelerated catalyst design applications, supporting seamless integration across cross-disciplinary studies.
title AceWGS: An LLM-Aided Framework to Accelerate Catalyst Design for Water-Gas Shift Reactions
topic Computation and Language
Artificial Intelligence
url https://arxiv.org/abs/2503.05607