Kagome goldene with flat bands and Dirac nodal line fermions via line-graph epitaxy

Fuente: arXiv
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Autores principales: Tian, Qiwei, Vishkayi, Sahar Izadi, Zhang, Chen, Zeng, Jiang, Li, Bo, Zhang, Li, Yin, Long-Jing, Tian, Yuan, Tagani, Meysam Bagheri, Zhang, Lijie, Qin, Zhihui
Formato: Preprint
Publicado: 2025
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author Tian, Qiwei
Vishkayi, Sahar Izadi
Zhang, Chen
Zeng, Jiang
Li, Bo
Zhang, Li
Yin, Long-Jing
Tian, Yuan
Tagani, Meysam Bagheri
Zhang, Lijie
Qin, Zhihui
author_facet Tian, Qiwei
Vishkayi, Sahar Izadi
Zhang, Chen
Zeng, Jiang
Li, Bo
Zhang, Li
Yin, Long-Jing
Tian, Yuan
Tagani, Meysam Bagheri
Zhang, Lijie
Qin, Zhihui
contents The kagome lattice has emerged as a promising platform for investigating exotic quantum phases. However, achieving a single-atomic-layer kagome lattice in elemental materials remains a significant challenge. Here, we introduce line-graph epitaxy, a novel approach that enables the atomic-scale synthesis of goldene, a monolayer of elemental gold atoms arranged in a kagome lattice. Through scanning tunneling microscopy/spectroscopy (STM/STS), and density functional theory (DFT) calculations, we demonstrate the formation of kagome goldene, featuring a flat band with a van Hove singularity approximately 1.1 eV below the Fermi level, signaling strong electron correlation effects. Notably, the flat band is disrupted at the zigzag edges of goldene nanoflakes, revealing substantial edge effects. Furthermore, our calculations show that weak interlayer interactions between goldene and the underlying Au2Ge substrate generate dual Dirac nodal lines through a proximity effect. These findings offer not only a novel strategy for constructing elemental kagome lattices, but also a generalizable framework for fabricating and controlling line-graph materials. This research advances the exploration of quantum phases driven by strong correlations and the design of materials for next-generation quantum technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2503_07945
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Kagome goldene with flat bands and Dirac nodal line fermions via line-graph epitaxy
Tian, Qiwei
Vishkayi, Sahar Izadi
Zhang, Chen
Zeng, Jiang
Li, Bo
Zhang, Li
Yin, Long-Jing
Tian, Yuan
Tagani, Meysam Bagheri
Zhang, Lijie
Qin, Zhihui
Mesoscale and Nanoscale Physics
Materials Science
The kagome lattice has emerged as a promising platform for investigating exotic quantum phases. However, achieving a single-atomic-layer kagome lattice in elemental materials remains a significant challenge. Here, we introduce line-graph epitaxy, a novel approach that enables the atomic-scale synthesis of goldene, a monolayer of elemental gold atoms arranged in a kagome lattice. Through scanning tunneling microscopy/spectroscopy (STM/STS), and density functional theory (DFT) calculations, we demonstrate the formation of kagome goldene, featuring a flat band with a van Hove singularity approximately 1.1 eV below the Fermi level, signaling strong electron correlation effects. Notably, the flat band is disrupted at the zigzag edges of goldene nanoflakes, revealing substantial edge effects. Furthermore, our calculations show that weak interlayer interactions between goldene and the underlying Au2Ge substrate generate dual Dirac nodal lines through a proximity effect. These findings offer not only a novel strategy for constructing elemental kagome lattices, but also a generalizable framework for fabricating and controlling line-graph materials. This research advances the exploration of quantum phases driven by strong correlations and the design of materials for next-generation quantum technologies.
title Kagome goldene with flat bands and Dirac nodal line fermions via line-graph epitaxy
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2503.07945