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| Main Authors: | , , , , |
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| Format: | Preprint |
| Published: |
2025
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| Subjects: | |
| Online Access: | https://arxiv.org/abs/2503.08058 |
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| _version_ | 1866917956604133376 |
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| author | Nomoto, Tetsuya Kikkawa, Akiko Nakazawa, Kazuki Yamaguchi, Terufumi Kagawa, Fumitaka |
| author_facet | Nomoto, Tetsuya Kikkawa, Akiko Nakazawa, Kazuki Yamaguchi, Terufumi Kagawa, Fumitaka |
| contents | The nonlinear thermoelectric effect is a key factor for realising unconventional thermoelectric phenomena, such as heat rectification and power generation using thermal fluctuations. Recent theoretical advances have indicated that chiral materials can host a variety of exotic nonlinear thermoelectric transport arising from inversion-symmetry breaking. However, experimental demonstration has yet to be achieved. Here, we report the observation of the nonlinear chiral thermoelectric Hall effect in chiral tellurium at room temperature, where a voltage is generated as a cross product of the temperature gradient and electric field. The resulting thermoelectric Hall voltage is on the order of μV, consistent with the prediction from the ab initio calculation. Furthermore, the sign of the thermoelectric Hall voltage is reversed depending on the crystal chirality, demonstrating a novel functionality of sign control of the thermoelectric effect by the chirality degrees of freedom. Our findings reveal the potential of chiral systems as nonlinear thermoelectric materials for advanced thermal management and energy harvesting. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2503_08058 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Observation of the nonlinear chiral thermoelectric Hall effect in tellurium Nomoto, Tetsuya Kikkawa, Akiko Nakazawa, Kazuki Yamaguchi, Terufumi Kagawa, Fumitaka Mesoscale and Nanoscale Physics Materials Science The nonlinear thermoelectric effect is a key factor for realising unconventional thermoelectric phenomena, such as heat rectification and power generation using thermal fluctuations. Recent theoretical advances have indicated that chiral materials can host a variety of exotic nonlinear thermoelectric transport arising from inversion-symmetry breaking. However, experimental demonstration has yet to be achieved. Here, we report the observation of the nonlinear chiral thermoelectric Hall effect in chiral tellurium at room temperature, where a voltage is generated as a cross product of the temperature gradient and electric field. The resulting thermoelectric Hall voltage is on the order of μV, consistent with the prediction from the ab initio calculation. Furthermore, the sign of the thermoelectric Hall voltage is reversed depending on the crystal chirality, demonstrating a novel functionality of sign control of the thermoelectric effect by the chirality degrees of freedom. Our findings reveal the potential of chiral systems as nonlinear thermoelectric materials for advanced thermal management and energy harvesting. |
| title | Observation of the nonlinear chiral thermoelectric Hall effect in tellurium |
| topic | Mesoscale and Nanoscale Physics Materials Science |
| url | https://arxiv.org/abs/2503.08058 |