Fluence dependent delay of Ni in an FeNi alloy supports an exchange based origin

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Auteurs principaux: Jana, Somnath, Knut, Ronny, Singh, Puloma, Yao, Kelvin, Tzschaschel, Christian, Richter, Johanna, Schick, Daniel, Sommer, Denny, Engel, Dieter, Karis, Olof, Schmising, Clemens von Korff, Eisebitt, Stefan
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Publié: 2025
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author Jana, Somnath
Knut, Ronny
Singh, Puloma
Yao, Kelvin
Tzschaschel, Christian
Richter, Johanna
Schick, Daniel
Sommer, Denny
Engel, Dieter
Karis, Olof
Schmising, Clemens von Korff
Eisebitt, Stefan
author_facet Jana, Somnath
Knut, Ronny
Singh, Puloma
Yao, Kelvin
Tzschaschel, Christian
Richter, Johanna
Schick, Daniel
Sommer, Denny
Engel, Dieter
Karis, Olof
Schmising, Clemens von Korff
Eisebitt, Stefan
contents The delayed demagnetization in Ni relative to Fe in the ultrafast demagnetization studies in FeNi alloy has led to two competing theoretical explanations: The Inhomogeneous Magnon Generation (IMG) and the Optically Induced Spin Transfer (OISTR) model. The IMG attributes the delay to the preferential magnon generation at the Fe sites and its subsequent propagation to Ni, while OISTR proposes direct spin transfer from Ni to Fe. In this study, we employ element-resolved extreme ultraviolet spectroscopy to investigate the effect of excitation strength on this delay, aiming to resolve the controversy. The data indicate a significant reduction in the delay with increasing fluence, which is inconsistent with the theoretical predictions of OISTR. These findings, in conjunction with the observation of a saturation of Fe demagnetization at the onset of Ni demagnetization, indicate that a spin-wave instability within the IMG framework may provide a potential explanation for the experimental results.
format Preprint
id arxiv_https___arxiv_org_abs_2503_08811
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Fluence dependent delay of Ni in an FeNi alloy supports an exchange based origin
Jana, Somnath
Knut, Ronny
Singh, Puloma
Yao, Kelvin
Tzschaschel, Christian
Richter, Johanna
Schick, Daniel
Sommer, Denny
Engel, Dieter
Karis, Olof
Schmising, Clemens von Korff
Eisebitt, Stefan
Materials Science
The delayed demagnetization in Ni relative to Fe in the ultrafast demagnetization studies in FeNi alloy has led to two competing theoretical explanations: The Inhomogeneous Magnon Generation (IMG) and the Optically Induced Spin Transfer (OISTR) model. The IMG attributes the delay to the preferential magnon generation at the Fe sites and its subsequent propagation to Ni, while OISTR proposes direct spin transfer from Ni to Fe. In this study, we employ element-resolved extreme ultraviolet spectroscopy to investigate the effect of excitation strength on this delay, aiming to resolve the controversy. The data indicate a significant reduction in the delay with increasing fluence, which is inconsistent with the theoretical predictions of OISTR. These findings, in conjunction with the observation of a saturation of Fe demagnetization at the onset of Ni demagnetization, indicate that a spin-wave instability within the IMG framework may provide a potential explanation for the experimental results.
title Fluence dependent delay of Ni in an FeNi alloy supports an exchange based origin
topic Materials Science
url https://arxiv.org/abs/2503.08811