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Main Authors: Bhuiyan, Mohammad T. H., Li, Qile, Blyth, James, Lee, Ji-Eun, Denlinger, Jonathan, Sánchez-Barriga, Jaime, Fedorov, Alexander, Tadich, Anton, Reinks, Emile, Mo, Sung-Kwan, Fedorov, Alexei, Clark, Oliver J., Edmonds, Mark T.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2503.10979
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author Bhuiyan, Mohammad T. H.
Li, Qile
Blyth, James
Lee, Ji-Eun
Denlinger, Jonathan
Sánchez-Barriga, Jaime
Fedorov, Alexander
Tadich, Anton
Reinks, Emile
Mo, Sung-Kwan
Fedorov, Alexei
Clark, Oliver J.
Edmonds, Mark T.
author_facet Bhuiyan, Mohammad T. H.
Li, Qile
Blyth, James
Lee, Ji-Eun
Denlinger, Jonathan
Sánchez-Barriga, Jaime
Fedorov, Alexander
Tadich, Anton
Reinks, Emile
Mo, Sung-Kwan
Fedorov, Alexei
Clark, Oliver J.
Edmonds, Mark T.
contents Quantum materials combining magnetism and topological fermions are a key platform for low-energy electronics, spintronics, and quantum phases that break time-reversal symmetry (TRS), such as the quantum anomalous Hall effect (QAHE). Coupling a topological insulator to a magnetic material allows proximity magnetization with the potential to achieve these phases at elevated temperatures. One potential architecture for realizing QAHE at elevated temperature is a heterostructure comprising two single-septuple layers (1SL) of MnBi2Te4 (a 2D ferromagnetic insulator) with four-quintuple layer (4QL) Bi2Te3 in the middle. However, the origin of this gap has not yet been explicitly determined, as there are other non-magnetic mechanisms that have been shown to produce bandgaps in similar systems. Here, through spin- and angle-resolved photoemission, the magnetic nature of the gap opening is investigated to demonstrates direct control of the spin state via small magnetic fields and confirm the magnetic origin of the gap through spin splitting and broken TRS. Furthermore, the hallmark chiral spin texture of non-magnetic topological insulators is preserved away from the Γ-point, despite the large 72+/-10 meV exchange gap at the Dirac point. The robust magnetic gap and controllable spin texture hold significant promise for future technologies requiring both magnetic properties and topological protection.
format Preprint
id arxiv_https___arxiv_org_abs_2503_10979
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spin Texture Control and Magnetic Gap Engineering in a Ferromagnetic Insulator-Topological Insulator Sandwiched Heterostructure
Bhuiyan, Mohammad T. H.
Li, Qile
Blyth, James
Lee, Ji-Eun
Denlinger, Jonathan
Sánchez-Barriga, Jaime
Fedorov, Alexander
Tadich, Anton
Reinks, Emile
Mo, Sung-Kwan
Fedorov, Alexei
Clark, Oliver J.
Edmonds, Mark T.
Materials Science
Quantum materials combining magnetism and topological fermions are a key platform for low-energy electronics, spintronics, and quantum phases that break time-reversal symmetry (TRS), such as the quantum anomalous Hall effect (QAHE). Coupling a topological insulator to a magnetic material allows proximity magnetization with the potential to achieve these phases at elevated temperatures. One potential architecture for realizing QAHE at elevated temperature is a heterostructure comprising two single-septuple layers (1SL) of MnBi2Te4 (a 2D ferromagnetic insulator) with four-quintuple layer (4QL) Bi2Te3 in the middle. However, the origin of this gap has not yet been explicitly determined, as there are other non-magnetic mechanisms that have been shown to produce bandgaps in similar systems. Here, through spin- and angle-resolved photoemission, the magnetic nature of the gap opening is investigated to demonstrates direct control of the spin state via small magnetic fields and confirm the magnetic origin of the gap through spin splitting and broken TRS. Furthermore, the hallmark chiral spin texture of non-magnetic topological insulators is preserved away from the Γ-point, despite the large 72+/-10 meV exchange gap at the Dirac point. The robust magnetic gap and controllable spin texture hold significant promise for future technologies requiring both magnetic properties and topological protection.
title Spin Texture Control and Magnetic Gap Engineering in a Ferromagnetic Insulator-Topological Insulator Sandwiched Heterostructure
topic Materials Science
url https://arxiv.org/abs/2503.10979