Fragility and thermal expansion control crystal melting and the glass transition

Fuente: arXiv
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Main Authors: Zaccone, Alessio, Samwer, Konrad
Format: Preprint
Published: 2025
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author Zaccone, Alessio
Samwer, Konrad
author_facet Zaccone, Alessio
Samwer, Konrad
contents Analytical relations for the glass transition temperature, $T_g$, and the crystal melting temperature, $T_m$, are developed on the basis of nonaffine lattice dynamics. The proposed relations explain: (i) the seemingly universal factor of $\approx 2/3$ difference between glass transition temperature and melting temperature of the corresponding crystal, and (ii) the recent empirical discovery that both $T_g$ and $T_m$ are proportional to the liquid fragility $m$ divided by the thermal expansion coefficient $α$ of the solid.
format Preprint
id arxiv_https___arxiv_org_abs_2503_13270
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Fragility and thermal expansion control crystal melting and the glass transition
Zaccone, Alessio
Samwer, Konrad
Soft Condensed Matter
Disordered Systems and Neural Networks
Materials Science
Statistical Mechanics
Chemical Physics
Analytical relations for the glass transition temperature, $T_g$, and the crystal melting temperature, $T_m$, are developed on the basis of nonaffine lattice dynamics. The proposed relations explain: (i) the seemingly universal factor of $\approx 2/3$ difference between glass transition temperature and melting temperature of the corresponding crystal, and (ii) the recent empirical discovery that both $T_g$ and $T_m$ are proportional to the liquid fragility $m$ divided by the thermal expansion coefficient $α$ of the solid.
title Fragility and thermal expansion control crystal melting and the glass transition
topic Soft Condensed Matter
Disordered Systems and Neural Networks
Materials Science
Statistical Mechanics
Chemical Physics
url https://arxiv.org/abs/2503.13270