Magnetoelastic coupling in intercalated transition metal dichalcogenides
Fuente:
arXiv
Saved in:
| Main Authors: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
|---|---|
| Format: | Preprint |
| Published: |
2025
|
| Subjects: | |
| Online Access: | |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1866908273677959168 |
|---|---|
| author | Kar, A. Basak, R. Li, Xue Korshunov, A. Subires, D. Phillips, J. Lim, C. -Y. Zhou, Feng Song, Linxuan Wang, Wenhong Lau, Yong-Chang Garbarino, G. Gargiani, P. Zhao, Y. Plueckthun, C. Francoual, S. Jana, A. Vobornik, I. Valla, T. Rajapitamahuni, A. Analytis, James G. Birgeneau, Robert J. Vescovo, E. Bosak, A. Dai, J. Tallarida, M. Frano, A. Pardo, V. Wu, S. Blanco-Canosa, S. |
| author_facet | Kar, A. Basak, R. Li, Xue Korshunov, A. Subires, D. Phillips, J. Lim, C. -Y. Zhou, Feng Song, Linxuan Wang, Wenhong Lau, Yong-Chang Garbarino, G. Gargiani, P. Zhao, Y. Plueckthun, C. Francoual, S. Jana, A. Vobornik, I. Valla, T. Rajapitamahuni, A. Analytis, James G. Birgeneau, Robert J. Vescovo, E. Bosak, A. Dai, J. Tallarida, M. Frano, A. Pardo, V. Wu, S. Blanco-Canosa, S. |
| contents | The large van der Waals gap in transition metal dichalcogenides (TMDs) offers an avenue to host external metal atoms that modify the ground state of these 2D materials. Here, we experimentally and theoretically address the charge correlations in a family of intercalated TMDs. While short-range charge fluctuations develop in Co$_{1/3}$TaS$_{2}$ and Fe$_{1/3}$TaS$_{2}$, long-range charge order switches-on in Fe$_{1/3}$NbS$_{2}$ driven by the interplay of magnetic order and lattice degrees of freedom. The magnetoelastic coupling is demonstrated in Fe$_{1/3}$NbS$_{2}$ by the enhancement of the charge modulations upon magnetic field below T$_\mathrm{N}$, although Density Functional Perturbation Theory (DFPT) calculations predict negligible electron(spin)-phonon coupling. Furthermore, we show that Co-intercalated TaS$_2$ displays a kagome-like Fermi surface, hence opening the path to engineer electronic band structures and study the entanglement of spin, charge, and spin-phonon mechanisms in the large family of intercalated TMDs. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2503_14444 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Magnetoelastic coupling in intercalated transition metal dichalcogenides Kar, A. Basak, R. Li, Xue Korshunov, A. Subires, D. Phillips, J. Lim, C. -Y. Zhou, Feng Song, Linxuan Wang, Wenhong Lau, Yong-Chang Garbarino, G. Gargiani, P. Zhao, Y. Plueckthun, C. Francoual, S. Jana, A. Vobornik, I. Valla, T. Rajapitamahuni, A. Analytis, James G. Birgeneau, Robert J. Vescovo, E. Bosak, A. Dai, J. Tallarida, M. Frano, A. Pardo, V. Wu, S. Blanco-Canosa, S. Strongly Correlated Electrons Materials Science The large van der Waals gap in transition metal dichalcogenides (TMDs) offers an avenue to host external metal atoms that modify the ground state of these 2D materials. Here, we experimentally and theoretically address the charge correlations in a family of intercalated TMDs. While short-range charge fluctuations develop in Co$_{1/3}$TaS$_{2}$ and Fe$_{1/3}$TaS$_{2}$, long-range charge order switches-on in Fe$_{1/3}$NbS$_{2}$ driven by the interplay of magnetic order and lattice degrees of freedom. The magnetoelastic coupling is demonstrated in Fe$_{1/3}$NbS$_{2}$ by the enhancement of the charge modulations upon magnetic field below T$_\mathrm{N}$, although Density Functional Perturbation Theory (DFPT) calculations predict negligible electron(spin)-phonon coupling. Furthermore, we show that Co-intercalated TaS$_2$ displays a kagome-like Fermi surface, hence opening the path to engineer electronic band structures and study the entanglement of spin, charge, and spin-phonon mechanisms in the large family of intercalated TMDs. |
| title | Magnetoelastic coupling in intercalated transition metal dichalcogenides |
| topic | Strongly Correlated Electrons Materials Science |
| url | https://arxiv.org/abs/2503.14444 |