Electrically switchable non-relativistic Zeeman spin splittings in collinear antiferromagnets

Fuente: arXiv
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Auteurs principaux: Yu, Longju, Zhao, Hong Jian, Bellaiche, Laurent, Ma, Yanming
Format: Preprint
Publié: 2025
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author Yu, Longju
Zhao, Hong Jian
Bellaiche, Laurent
Ma, Yanming
author_facet Yu, Longju
Zhao, Hong Jian
Bellaiche, Laurent
Ma, Yanming
contents Magnetic or electrical manipulation of electronic spin is elementary for spin-based logic, computing, and memory, where the latter is a low-power manipulation scheme. Rashba-like spin splittings stemming from spin-orbit interaction (SOI) enable electric-field manipulation of spin, but the relativistic SOI causes spin relaxations and yields dissipative transport of spin-encoded information. Recent works suggest the occurrence of electric-field switchable non-relativistic Zeeman spin splittings (NRZSSs) in collinear antiferromagnets -- allowing for electrical manipulation of spin in the non-relativistic regime; yet, a theory elucidating the mechanisms for these NRZSSs and guiding the materials discovery remains missing. Here, we develop such a theory by analyzing the symmetries of spin point groups. We highlight the linear magnetoelectric and bilinear piezomagnetoelectric mechanisms for NRZSSs that depend linearly on electric field and are electrically switchable. First-principles calculations further confirm that FeOOH and NaMnP showcase such NRZSSs. Our theory provides guidelines for discovering light-element collinear antiferromagnets with electrically switchable NRZSSs, which are promising for the design of high-performance spin-based devices.
format Preprint
id arxiv_https___arxiv_org_abs_2503_15215
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Electrically switchable non-relativistic Zeeman spin splittings in collinear antiferromagnets
Yu, Longju
Zhao, Hong Jian
Bellaiche, Laurent
Ma, Yanming
Materials Science
Magnetic or electrical manipulation of electronic spin is elementary for spin-based logic, computing, and memory, where the latter is a low-power manipulation scheme. Rashba-like spin splittings stemming from spin-orbit interaction (SOI) enable electric-field manipulation of spin, but the relativistic SOI causes spin relaxations and yields dissipative transport of spin-encoded information. Recent works suggest the occurrence of electric-field switchable non-relativistic Zeeman spin splittings (NRZSSs) in collinear antiferromagnets -- allowing for electrical manipulation of spin in the non-relativistic regime; yet, a theory elucidating the mechanisms for these NRZSSs and guiding the materials discovery remains missing. Here, we develop such a theory by analyzing the symmetries of spin point groups. We highlight the linear magnetoelectric and bilinear piezomagnetoelectric mechanisms for NRZSSs that depend linearly on electric field and are electrically switchable. First-principles calculations further confirm that FeOOH and NaMnP showcase such NRZSSs. Our theory provides guidelines for discovering light-element collinear antiferromagnets with electrically switchable NRZSSs, which are promising for the design of high-performance spin-based devices.
title Electrically switchable non-relativistic Zeeman spin splittings in collinear antiferromagnets
topic Materials Science
url https://arxiv.org/abs/2503.15215