Active wetting transitions induced by rotational noise at solid interfaces

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Hauptverfasser: Das, Suchismita, Chelakkot, Raghunath
Format: Preprint
Veröffentlicht: 2025
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author Das, Suchismita
Chelakkot, Raghunath
author_facet Das, Suchismita
Chelakkot, Raghunath
contents We investigate the wetting transitions displayed by the collection of active Brownian particles (ABPs) confined within rigid, impenetrable, flat walls. In our computational study using Brownian dynamics simulations, the wall-particle interactions are implemented with a short-range repulsive potential. An enhanced rotational diffusion at the walls is used as a control parameter for wetting transitions. Increasing the wall rotational diffusion destabilizes complete wetting, and the aggregate shows morphological transitions. We observe a sequence of morphological transitions with an increase in wall rotational diffusion: symmetric complete wetting (SCW), asymmetric complete wetting (ACW), partial wetting (PW) with droplet formation, and drying. In the PW state, we compute the contact angle as a function of activity and rotational noise. Our analysis indicates that these transitions are linked to enhanced kinetic energy fluctuations of particles and bubble formations in the dense state. We further characterize the nature of these transitions by systematically analyzing an order parameter. Our work shows that modifying local reorientation rates alone is sufficient to induce wetting transitions in active systems.
format Preprint
id arxiv_https___arxiv_org_abs_2503_15476
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Active wetting transitions induced by rotational noise at solid interfaces
Das, Suchismita
Chelakkot, Raghunath
Soft Condensed Matter
We investigate the wetting transitions displayed by the collection of active Brownian particles (ABPs) confined within rigid, impenetrable, flat walls. In our computational study using Brownian dynamics simulations, the wall-particle interactions are implemented with a short-range repulsive potential. An enhanced rotational diffusion at the walls is used as a control parameter for wetting transitions. Increasing the wall rotational diffusion destabilizes complete wetting, and the aggregate shows morphological transitions. We observe a sequence of morphological transitions with an increase in wall rotational diffusion: symmetric complete wetting (SCW), asymmetric complete wetting (ACW), partial wetting (PW) with droplet formation, and drying. In the PW state, we compute the contact angle as a function of activity and rotational noise. Our analysis indicates that these transitions are linked to enhanced kinetic energy fluctuations of particles and bubble formations in the dense state. We further characterize the nature of these transitions by systematically analyzing an order parameter. Our work shows that modifying local reorientation rates alone is sufficient to induce wetting transitions in active systems.
title Active wetting transitions induced by rotational noise at solid interfaces
topic Soft Condensed Matter
url https://arxiv.org/abs/2503.15476