Optical control of the moiré twist angle

Fuente: arXiv
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Autori principali: He, Zhiren, Jharapla, Prathap Kumar, Leconte, Nicolas, Jung, Jeil, Khalsa, Guru
Natura: Preprint
Pubblicazione: 2025
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author He, Zhiren
Jharapla, Prathap Kumar
Leconte, Nicolas
Jung, Jeil
Khalsa, Guru
author_facet He, Zhiren
Jharapla, Prathap Kumar
Leconte, Nicolas
Jung, Jeil
Khalsa, Guru
contents In this theoretical work, we propose an all-optical method for fast, precise manipulation of two-dimensional multilayers by transferring orbital angular momentum from phase-structured light (e.g. vortex beams) to a 2D material flake. We model the light-matter interaction, analyze the twist dynamics, and develop a phase diagram for optical twists by mapping the system onto an impulsively forced nonlinear pendulum. Our findings reveal rich dynamical responses spanning single- and multi-pulse twist angle control to (quasi)stable dynamical trajectories, and suggest a pathway for all-optical measurement of the twist potential energy. Aided by classical potential estimates for the interlayer energy and numerical simulation, we demonstrate the feasibility of this approach with hexagonal boron nitride bilayers and extend the results to dichalcogenides with first-principles calculations. These results can be generalized to other 2D multilayers, paving the way for scalable and customizable moiré electronics and photonics.
format Preprint
id arxiv_https___arxiv_org_abs_2503_15882
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Optical control of the moiré twist angle
He, Zhiren
Jharapla, Prathap Kumar
Leconte, Nicolas
Jung, Jeil
Khalsa, Guru
Materials Science
Optics
In this theoretical work, we propose an all-optical method for fast, precise manipulation of two-dimensional multilayers by transferring orbital angular momentum from phase-structured light (e.g. vortex beams) to a 2D material flake. We model the light-matter interaction, analyze the twist dynamics, and develop a phase diagram for optical twists by mapping the system onto an impulsively forced nonlinear pendulum. Our findings reveal rich dynamical responses spanning single- and multi-pulse twist angle control to (quasi)stable dynamical trajectories, and suggest a pathway for all-optical measurement of the twist potential energy. Aided by classical potential estimates for the interlayer energy and numerical simulation, we demonstrate the feasibility of this approach with hexagonal boron nitride bilayers and extend the results to dichalcogenides with first-principles calculations. These results can be generalized to other 2D multilayers, paving the way for scalable and customizable moiré electronics and photonics.
title Optical control of the moiré twist angle
topic Materials Science
Optics
url https://arxiv.org/abs/2503.15882