Electronic structure of a layered altermagnetic compound CoNb4Se8

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Hauptverfasser: Sakhya, Anup Pradhan, Mondal, Mazharul Islam, Sprague, Milo, Regmi, Resham Babu, Kumay, Arun K, Sheokand, Himanshu, Mazin, Igor. I., Ghimire, Nirmal J., Neupane, Madhab
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Veröffentlicht: 2025
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author Sakhya, Anup Pradhan
Mondal, Mazharul Islam
Sprague, Milo
Regmi, Resham Babu
Kumay, Arun K
Sheokand, Himanshu
Mazin, Igor. I.
Ghimire, Nirmal J.
Neupane, Madhab
author_facet Sakhya, Anup Pradhan
Mondal, Mazharul Islam
Sprague, Milo
Regmi, Resham Babu
Kumay, Arun K
Sheokand, Himanshu
Mazin, Igor. I.
Ghimire, Nirmal J.
Neupane, Madhab
contents Recently, there has been a growing interest in altermagnetism, a novel form of magnetism, characterized by unique spin-splitting even in the absence of both net magnetic moments and spin-orbit coupling. Despite numerous theoretical predictions, experimental evidence of such spin-splitting in real materials remains limited. In this study, we use angle-resolved photoemission spectroscopy (ARPES) combined with density functional theory (DFT) calculations to investigate the electronic band structure of the altermagnet candidate CoNb4Se8. This material features an ordered sublattice of intercalated Co atoms within NbSe2 layers. Magnetization and electrical resistivity measurements reveal the onset of antiferromagnetism below 168 K. Temperature dependent ARPES data, supported by DFT calculations, uncover spin split bands along the MGM high-symmetry direction. The observation of spin splitting in this high temperature altermagnet opens new avenues for exploring its electronic properties and potential applications in spintronic technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2503_16670
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Electronic structure of a layered altermagnetic compound CoNb4Se8
Sakhya, Anup Pradhan
Mondal, Mazharul Islam
Sprague, Milo
Regmi, Resham Babu
Kumay, Arun K
Sheokand, Himanshu
Mazin, Igor. I.
Ghimire, Nirmal J.
Neupane, Madhab
Mesoscale and Nanoscale Physics
Materials Science
Recently, there has been a growing interest in altermagnetism, a novel form of magnetism, characterized by unique spin-splitting even in the absence of both net magnetic moments and spin-orbit coupling. Despite numerous theoretical predictions, experimental evidence of such spin-splitting in real materials remains limited. In this study, we use angle-resolved photoemission spectroscopy (ARPES) combined with density functional theory (DFT) calculations to investigate the electronic band structure of the altermagnet candidate CoNb4Se8. This material features an ordered sublattice of intercalated Co atoms within NbSe2 layers. Magnetization and electrical resistivity measurements reveal the onset of antiferromagnetism below 168 K. Temperature dependent ARPES data, supported by DFT calculations, uncover spin split bands along the MGM high-symmetry direction. The observation of spin splitting in this high temperature altermagnet opens new avenues for exploring its electronic properties and potential applications in spintronic technologies.
title Electronic structure of a layered altermagnetic compound CoNb4Se8
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2503.16670