Nanometric skyrmion lattice from anisotropic exchange interactions in a centrosymmetric host

Fuente: arXiv
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Main Authors: Hirschberger, Max, Hayami, Satoru, Tokura, Yoshinori
Format: Preprint
Published: 2025
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_version_ 1866912290497888256
author Hirschberger, Max
Hayami, Satoru
Tokura, Yoshinori
author_facet Hirschberger, Max
Hayami, Satoru
Tokura, Yoshinori
contents Skyrmion formation in centrosymmetric magnets without Dzyaloshinskii-Moriya interactions was originally predicted from unbiased numerical techniques. However, no attempt has yet been made, by comparison to a real material, to determine the salient interaction terms and model parameters driving spin-vortex formation. We identify a Hamiltonian with anisotropic exchange couplings, local ion anisotropy, and four-spin interactions, which is generally applicable to this class of compounds. In the representative system Gd3Ru4Al12, anisotropic exchange drives a fragile balance between helical, skyrmion lattice, and transverse conical (cycloidal) orders. The model is severely constrained by the experimentally observed collapse of the SkL with a small in-plane magnetic field. For the zero-field helical state, we further anticipate that spins can be easily rotated out of the spiral plane by a tilted magnetic field or applied current.
format Preprint
id arxiv_https___arxiv_org_abs_2503_18632
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Nanometric skyrmion lattice from anisotropic exchange interactions in a centrosymmetric host
Hirschberger, Max
Hayami, Satoru
Tokura, Yoshinori
Strongly Correlated Electrons
Materials Science
Skyrmion formation in centrosymmetric magnets without Dzyaloshinskii-Moriya interactions was originally predicted from unbiased numerical techniques. However, no attempt has yet been made, by comparison to a real material, to determine the salient interaction terms and model parameters driving spin-vortex formation. We identify a Hamiltonian with anisotropic exchange couplings, local ion anisotropy, and four-spin interactions, which is generally applicable to this class of compounds. In the representative system Gd3Ru4Al12, anisotropic exchange drives a fragile balance between helical, skyrmion lattice, and transverse conical (cycloidal) orders. The model is severely constrained by the experimentally observed collapse of the SkL with a small in-plane magnetic field. For the zero-field helical state, we further anticipate that spins can be easily rotated out of the spiral plane by a tilted magnetic field or applied current.
title Nanometric skyrmion lattice from anisotropic exchange interactions in a centrosymmetric host
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2503.18632