Quasiparticle Spectroscopy of Chiral Charge Order

Fuente: arXiv
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Autores principales: Zheng, Jiangchang, Chen, Caiyun, Pan, Gaopei, Zhang, Xu, Chen, Chen, Da Liao, Yuan, Pokharel, Ganesh, Salinas, Andrea Capa, Wei, Yizhou, Po, Hoi Chun, Pan, Ding, Wilson, Stephen D., Meng, Zi Yang, Jäck, Berthold
Formato: Preprint
Publicado: 2025
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author Zheng, Jiangchang
Chen, Caiyun
Pan, Gaopei
Zhang, Xu
Chen, Chen
Da Liao, Yuan
Pokharel, Ganesh
Salinas, Andrea Capa
Wei, Yizhou
Po, Hoi Chun
Pan, Ding
Wilson, Stephen D.
Meng, Zi Yang
Jäck, Berthold
author_facet Zheng, Jiangchang
Chen, Caiyun
Pan, Gaopei
Zhang, Xu
Chen, Chen
Da Liao, Yuan
Pokharel, Ganesh
Salinas, Andrea Capa
Wei, Yizhou
Po, Hoi Chun
Pan, Ding
Wilson, Stephen D.
Meng, Zi Yang
Jäck, Berthold
contents Electronic interactions can give rise to novel charge density waves with unconventional ground states. Recent experiments report evidence for a chiral charge density wave (CDW) that breaks time-reversal symmetry in the kagome metals AV$_3$Sb$_5$ (A=K, Rb or Cs). Theoretical analyses propose a topologically nontrivial loop current phase that spontaneously breaks time-reversal symmetry as the favorable CDW ground state. However, spectroscopic insights into the quasiparticle excitations of chiral charge order in AV$_3$Sb$_5$ compounds are still missing and conflicting experimental results question the presence of a loop current phase. We employed individual magnetic atoms as local quantum sensors to examine the quasiparticle excitations of chiral charge order in CsV$_3$Sb$_5$ with the scanning tunneling microscope (STM). Our spectroscopic measurements show that the magnetic moment of Co induces a spatially-localized low-energy state in the CDW phase. The distinct spectral signatures of this state are consistent with theoretical expectations for the quasiparticle excitation of a loop current order parameter, while control experiment rule out alternative scenario. Our work provides unique insights into the ground state of chiral charge order in CsV$_3$Sb$_5$ and introduces a novel method to examine other topological states, such as the fractional Chern insulators, with the STM.
format Preprint
id arxiv_https___arxiv_org_abs_2503_19032
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Quasiparticle Spectroscopy of Chiral Charge Order
Zheng, Jiangchang
Chen, Caiyun
Pan, Gaopei
Zhang, Xu
Chen, Chen
Da Liao, Yuan
Pokharel, Ganesh
Salinas, Andrea Capa
Wei, Yizhou
Po, Hoi Chun
Pan, Ding
Wilson, Stephen D.
Meng, Zi Yang
Jäck, Berthold
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
Electronic interactions can give rise to novel charge density waves with unconventional ground states. Recent experiments report evidence for a chiral charge density wave (CDW) that breaks time-reversal symmetry in the kagome metals AV$_3$Sb$_5$ (A=K, Rb or Cs). Theoretical analyses propose a topologically nontrivial loop current phase that spontaneously breaks time-reversal symmetry as the favorable CDW ground state. However, spectroscopic insights into the quasiparticle excitations of chiral charge order in AV$_3$Sb$_5$ compounds are still missing and conflicting experimental results question the presence of a loop current phase. We employed individual magnetic atoms as local quantum sensors to examine the quasiparticle excitations of chiral charge order in CsV$_3$Sb$_5$ with the scanning tunneling microscope (STM). Our spectroscopic measurements show that the magnetic moment of Co induces a spatially-localized low-energy state in the CDW phase. The distinct spectral signatures of this state are consistent with theoretical expectations for the quasiparticle excitation of a loop current order parameter, while control experiment rule out alternative scenario. Our work provides unique insights into the ground state of chiral charge order in CsV$_3$Sb$_5$ and introduces a novel method to examine other topological states, such as the fractional Chern insulators, with the STM.
title Quasiparticle Spectroscopy of Chiral Charge Order
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2503.19032