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Main Authors: Zhang, Long, Jiang, Zhongzhu, Zhang, Yugang, Zhang, Jing, Wang, Aifeng, He, Mingquan, Sun, Yuping, Luo, Xuan, Chai, Yisheng
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2503.20261
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author Zhang, Long
Jiang, Zhongzhu
Zhang, Yugang
Zhang, Jing
Wang, Aifeng
He, Mingquan
Sun, Yuping
Luo, Xuan
Chai, Yisheng
author_facet Zhang, Long
Jiang, Zhongzhu
Zhang, Yugang
Zhang, Jing
Wang, Aifeng
He, Mingquan
Sun, Yuping
Luo, Xuan
Chai, Yisheng
contents Two-dimensional (2D) magnetic materials have attracted considerable interest owing to their potential applications in spintronics and fundamental investigations into low-dimensional magnetism. Cr2Te3, a quasi 2D non van der Waals magnet, exhibits a complex magnetic phase diagram due to competing magnetic interactions within and between layers. However, the precise nature and evolution of these magnetic phases remain unclear. Here, we utilize an ultrahigh-sensitive composite magnetoelectric technique, which probes the ac magnetostrictive coefficient, to systematically explore the temperature magnetic field phase diagram of Cr2Te3 single crystals. Our results reveal the coexistence of multiple magnetic phases, including canted ferromagnetic, antiferromagnetic, and paramagnetic states. Another canted ferromagnetic phase and a possible triple point have been proposed. The updated phase diagram provides deeper insights into the specific spin configurations associated with each phase. These findings also highlight the decoupled magnetic ordering between the Cr1/Cr3 layers and the Cr2 layer near the magnetic ordering temperature.
format Preprint
id arxiv_https___arxiv_org_abs_2503_20261
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Magnetic phase diagram of Cr2Te3 revisited by ac magnetostrictive coefficient
Zhang, Long
Jiang, Zhongzhu
Zhang, Yugang
Zhang, Jing
Wang, Aifeng
He, Mingquan
Sun, Yuping
Luo, Xuan
Chai, Yisheng
Materials Science
Strongly Correlated Electrons
Two-dimensional (2D) magnetic materials have attracted considerable interest owing to their potential applications in spintronics and fundamental investigations into low-dimensional magnetism. Cr2Te3, a quasi 2D non van der Waals magnet, exhibits a complex magnetic phase diagram due to competing magnetic interactions within and between layers. However, the precise nature and evolution of these magnetic phases remain unclear. Here, we utilize an ultrahigh-sensitive composite magnetoelectric technique, which probes the ac magnetostrictive coefficient, to systematically explore the temperature magnetic field phase diagram of Cr2Te3 single crystals. Our results reveal the coexistence of multiple magnetic phases, including canted ferromagnetic, antiferromagnetic, and paramagnetic states. Another canted ferromagnetic phase and a possible triple point have been proposed. The updated phase diagram provides deeper insights into the specific spin configurations associated with each phase. These findings also highlight the decoupled magnetic ordering between the Cr1/Cr3 layers and the Cr2 layer near the magnetic ordering temperature.
title Magnetic phase diagram of Cr2Te3 revisited by ac magnetostrictive coefficient
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2503.20261