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Main Authors: Catalan, G., Gruverman, A., Íñiguez-González, J., Meier, D., Trassin, M.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2503.20423
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author Catalan, G.
Gruverman, A.
Íñiguez-González, J.
Meier, D.
Trassin, M.
author_facet Catalan, G.
Gruverman, A.
Íñiguez-González, J.
Meier, D.
Trassin, M.
contents Antiferroelectrics attract broad attention due to their unusual physical characteristics, chief among which is the double-hysteresis loop that separates their antipolar ground state from the voltage-induced polar phase, which is promising for applications in energy storage and electrocaloric cooling. However, their defining features (antipolar ground state and double-hysteresis loops) are increasingly challenged: materials with non-collinear and/or hybrid polar-antipolar order have been discovered, and double-hysteresis has been realized in materials without a conventional antipolar ground state. These developments add to the intensifying interest in fundamental and practical aspects of antiferroelectrics, and call for a fresh look at antiferroelectricity. In this Perspective, we provide an updated and all-encompassing definition of antiferroelectricity, discuss material systems with new antipolar orders and/or engineered double hysteresis, and reflect on emergent properties and theoretical approaches. This work casts a bird's eye view on the rapidly evolving trends that are shaping up the research on ferroics with antipolar order.
format Preprint
id arxiv_https___arxiv_org_abs_2503_20423
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Switching on Antiferroelectrics
Catalan, G.
Gruverman, A.
Íñiguez-González, J.
Meier, D.
Trassin, M.
Materials Science
Antiferroelectrics attract broad attention due to their unusual physical characteristics, chief among which is the double-hysteresis loop that separates their antipolar ground state from the voltage-induced polar phase, which is promising for applications in energy storage and electrocaloric cooling. However, their defining features (antipolar ground state and double-hysteresis loops) are increasingly challenged: materials with non-collinear and/or hybrid polar-antipolar order have been discovered, and double-hysteresis has been realized in materials without a conventional antipolar ground state. These developments add to the intensifying interest in fundamental and practical aspects of antiferroelectrics, and call for a fresh look at antiferroelectricity. In this Perspective, we provide an updated and all-encompassing definition of antiferroelectricity, discuss material systems with new antipolar orders and/or engineered double hysteresis, and reflect on emergent properties and theoretical approaches. This work casts a bird's eye view on the rapidly evolving trends that are shaping up the research on ferroics with antipolar order.
title Switching on Antiferroelectrics
topic Materials Science
url https://arxiv.org/abs/2503.20423