Giant Spin Pumping at Polymer/Ferromagnet Interfaces for Hybrid Spintronic Devices

Fuente: arXiv
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Autori principali: Gaur, Shiva, Kumar, Akash, Bangar, Himanshu, Shashank, Utkarsh, Singh, Hukum, Dash, Saroj P., Raghav, Anubhav, Åkerman, Johan
Natura: Preprint
Pubblicazione: 2025
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author Gaur, Shiva
Kumar, Akash
Bangar, Himanshu
Shashank, Utkarsh
Singh, Hukum
Dash, Saroj P.
Raghav, Anubhav
Åkerman, Johan
author_facet Gaur, Shiva
Kumar, Akash
Bangar, Himanshu
Shashank, Utkarsh
Singh, Hukum
Dash, Saroj P.
Raghav, Anubhav
Åkerman, Johan
contents While the growing utilization of polymers in flexible electronic devices has sparked significant interest in polymer/metal interfaces, spintronic studies of such interfaces remain limited. Here, we systematically study spin pumping across a polymer/ferromagnet metal interface between hydrogen silsesquioxane (HSQ) oligomer layers ($t_\mathit{HSQ} = 30, 36, 48$ nm) and NiFe ($t_\mathit{NiFe} = 4, 5, 7, 10$ nm) thin films. Using ferromagnetic resonance measurements, we observe strong spin pumping (large linewidth broadening) and a giant spin mixing conductance, reaching 19.8~${\rm nm^{-2}}$ for HSQ = 48 nm, \emph{i.e.}~comparable to that of heavy metals. Our results suggest efficient spin transfer across the HSQ/NiFe interface, possibly originating from a combination of spin and orbital pumping, and provide valuable insights for designing self-powered and flexible spintronic devices utilizing polymers in combination with ferromagnetic materials.
format Preprint
id arxiv_https___arxiv_org_abs_2503_22623
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Giant Spin Pumping at Polymer/Ferromagnet Interfaces for Hybrid Spintronic Devices
Gaur, Shiva
Kumar, Akash
Bangar, Himanshu
Shashank, Utkarsh
Singh, Hukum
Dash, Saroj P.
Raghav, Anubhav
Åkerman, Johan
Mesoscale and Nanoscale Physics
While the growing utilization of polymers in flexible electronic devices has sparked significant interest in polymer/metal interfaces, spintronic studies of such interfaces remain limited. Here, we systematically study spin pumping across a polymer/ferromagnet metal interface between hydrogen silsesquioxane (HSQ) oligomer layers ($t_\mathit{HSQ} = 30, 36, 48$ nm) and NiFe ($t_\mathit{NiFe} = 4, 5, 7, 10$ nm) thin films. Using ferromagnetic resonance measurements, we observe strong spin pumping (large linewidth broadening) and a giant spin mixing conductance, reaching 19.8~${\rm nm^{-2}}$ for HSQ = 48 nm, \emph{i.e.}~comparable to that of heavy metals. Our results suggest efficient spin transfer across the HSQ/NiFe interface, possibly originating from a combination of spin and orbital pumping, and provide valuable insights for designing self-powered and flexible spintronic devices utilizing polymers in combination with ferromagnetic materials.
title Giant Spin Pumping at Polymer/Ferromagnet Interfaces for Hybrid Spintronic Devices
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2503.22623