Angle-Dependent Magnetoresistance Induced by Interface-Generated Spin Current in RuO$_2$/Permalloy Heterostructures

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Main Authors: Akashdeep, Akashdeep, Ababneh, Ewiese Mohammad, Schmitt, Christin, Galíndez-Ruales, Edgar, Fuhrmann, Felix, Kuschel, Timo, Kläui, Mathias, Amin, Vivek Pravin, Jakob, Gerhard
Format: Preprint
Published: 2025
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author Akashdeep, Akashdeep
Ababneh, Ewiese Mohammad
Schmitt, Christin
Galíndez-Ruales, Edgar
Fuhrmann, Felix
Kuschel, Timo
Kläui, Mathias
Amin, Vivek Pravin
Jakob, Gerhard
author_facet Akashdeep, Akashdeep
Ababneh, Ewiese Mohammad
Schmitt, Christin
Galíndez-Ruales, Edgar
Fuhrmann, Felix
Kuschel, Timo
Kläui, Mathias
Amin, Vivek Pravin
Jakob, Gerhard
contents Altermagnets, a recently discovered class of magnetic materials exhibiting ferromagnetic-like spin-split bands and antiferromagnetic-like compensated magnetic order, have attracted significant interest for next-generation spintronic applications. Ruthenium dioxide (RuO2) has emerged as a promising altermagnetic candidate due to its compensated antiparallel magnetic order and strong spin-split electronic bands. However, recent experimental and theoretical reports also suggest that RuO2 may be non-magnetic in its ground state, underscoring the need for deeper investigations into its magnetic character. Specifically, the (100)-oriented RuO2 films are expected to generate spin currents with transverse spin polarization parallel to the Néel vector. Here, we investigate magnetotransport in epitaxial RuO2/Permalloy (Py) heterostructures to examine spin Hall magnetoresistance and interfacial effects generated in such systems. Our measurements reveal a pronounced negative angular-dependent magnetoresistance for variation of magnetic field direction perpendicular to the charge current direction. Detailed temperature-, magnetic field-, and crystallographic orientation-dependent measurements indicate that interface-generated spin current (IGSC) at the RuO2/Py interface predominantly governs the observed magnetoresistance. This shows that strong interface effects dominate over possible altermagnetic contributions from RuO2. Our results show that the role of interface-generated spin currents is crucial and should not be overlooked in studies of altermagnetic systems. A critical step in this direction is disentangling interfacial from altermagnetic contributions. The insight into interfacial contributions from altermagnetic influences is essential for the advancement of RuO2 based spintronic memory and sensing applications.
format Preprint
id arxiv_https___arxiv_org_abs_2504_00230
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Angle-Dependent Magnetoresistance Induced by Interface-Generated Spin Current in RuO$_2$/Permalloy Heterostructures
Akashdeep, Akashdeep
Ababneh, Ewiese Mohammad
Schmitt, Christin
Galíndez-Ruales, Edgar
Fuhrmann, Felix
Kuschel, Timo
Kläui, Mathias
Amin, Vivek Pravin
Jakob, Gerhard
Mesoscale and Nanoscale Physics
Altermagnets, a recently discovered class of magnetic materials exhibiting ferromagnetic-like spin-split bands and antiferromagnetic-like compensated magnetic order, have attracted significant interest for next-generation spintronic applications. Ruthenium dioxide (RuO2) has emerged as a promising altermagnetic candidate due to its compensated antiparallel magnetic order and strong spin-split electronic bands. However, recent experimental and theoretical reports also suggest that RuO2 may be non-magnetic in its ground state, underscoring the need for deeper investigations into its magnetic character. Specifically, the (100)-oriented RuO2 films are expected to generate spin currents with transverse spin polarization parallel to the Néel vector. Here, we investigate magnetotransport in epitaxial RuO2/Permalloy (Py) heterostructures to examine spin Hall magnetoresistance and interfacial effects generated in such systems. Our measurements reveal a pronounced negative angular-dependent magnetoresistance for variation of magnetic field direction perpendicular to the charge current direction. Detailed temperature-, magnetic field-, and crystallographic orientation-dependent measurements indicate that interface-generated spin current (IGSC) at the RuO2/Py interface predominantly governs the observed magnetoresistance. This shows that strong interface effects dominate over possible altermagnetic contributions from RuO2. Our results show that the role of interface-generated spin currents is crucial and should not be overlooked in studies of altermagnetic systems. A critical step in this direction is disentangling interfacial from altermagnetic contributions. The insight into interfacial contributions from altermagnetic influences is essential for the advancement of RuO2 based spintronic memory and sensing applications.
title Angle-Dependent Magnetoresistance Induced by Interface-Generated Spin Current in RuO$_2$/Permalloy Heterostructures
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2504.00230