Polarization-dependent photocurrent in a quadrilateral-shaped bulk crystalline tellurium chip with near-infrared light excitation

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Main Authors: Munekata, Hiro, Kusuno, Gakuto, Miyazaki, Kohei, Satoh, Takuya
Format: Preprint
Published: 2025
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author Munekata, Hiro
Kusuno, Gakuto
Miyazaki, Kohei
Satoh, Takuya
author_facet Munekata, Hiro
Kusuno, Gakuto
Miyazaki, Kohei
Satoh, Takuya
contents We report the detection of zero-bias photocurrents induced by interband excitation using oblique near-infrared light (λ=0.780 μm) along the directions parallel and perpendicular to the helical axis in a millimeter-sized Te crystal. The photocurrent parallel to the helical axis exhibits a circular-polarization-dependent component, namely circular photogalvanic effect. We create a framework for estimating the gyrotropic photoconductivity tensor \b{eta}, the ratio between the circular-polarization-dependent photocurrent density and intensity of light, through which extrinsic \b{eta} values ranging from a few to a few tens of nA/W are obtained. Searching the \b{eta} values through existing literatures reveals that these values vary significantly with sample conditions, excitation wavelengths, and forms of crystallite samples. A particular interesting point found in our study is that the \b{eta} values for the interband excitation may be greater than those for intraband excitation as far as bulk Te is concerned.
format Preprint
id arxiv_https___arxiv_org_abs_2504_00413
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Polarization-dependent photocurrent in a quadrilateral-shaped bulk crystalline tellurium chip with near-infrared light excitation
Munekata, Hiro
Kusuno, Gakuto
Miyazaki, Kohei
Satoh, Takuya
Materials Science
We report the detection of zero-bias photocurrents induced by interband excitation using oblique near-infrared light (λ=0.780 μm) along the directions parallel and perpendicular to the helical axis in a millimeter-sized Te crystal. The photocurrent parallel to the helical axis exhibits a circular-polarization-dependent component, namely circular photogalvanic effect. We create a framework for estimating the gyrotropic photoconductivity tensor \b{eta}, the ratio between the circular-polarization-dependent photocurrent density and intensity of light, through which extrinsic \b{eta} values ranging from a few to a few tens of nA/W are obtained. Searching the \b{eta} values through existing literatures reveals that these values vary significantly with sample conditions, excitation wavelengths, and forms of crystallite samples. A particular interesting point found in our study is that the \b{eta} values for the interband excitation may be greater than those for intraband excitation as far as bulk Te is concerned.
title Polarization-dependent photocurrent in a quadrilateral-shaped bulk crystalline tellurium chip with near-infrared light excitation
topic Materials Science
url https://arxiv.org/abs/2504.00413