Driving collective current excitations using light: The two-time $GW$ approach

Fuente: arXiv
Gespeichert in:
Bibliographische Detailangaben
Hauptverfasser: Ong, Chin Shen, Golež, Denis, Rubio, Angel, Eriksson, Olle, Strand, Hugo U. R.
Format: Preprint
Veröffentlicht: 2025
Schlagworte:
Online-Zugang:
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
_version_ 1866916849510252544
author Ong, Chin Shen
Golež, Denis
Rubio, Angel
Eriksson, Olle
Strand, Hugo U. R.
author_facet Ong, Chin Shen
Golež, Denis
Rubio, Angel
Eriksson, Olle
Strand, Hugo U. R.
contents We identify a distinct transverse collective excitation, which we name the "curron", arising from current-current interactions in a driven quantum metal. Unlike plasmons, which involve longitudinal charge oscillations, currons are transverse current-density oscillations resulting from the interplay between the vector potential generated by the current and the external driving field. We demonstrate the emergence of this excitation in sodium metal by solving the Kadanoff-Baym equations on a complex time contour within the non-equilibrium two-time (TT) $GW$ formalism, marking, to our knowledge, the first TT-$GW$ calculation on a realistic material. We further show that two-time quantum memory effects leave measurable signatures: a pump-induced elevation in the baseline of the current-to-field response, potentially observable in polarization- and momentum-resolved conductivity experiments. By extracting effective resistive and memory coefficients from the TT-$GW$ dynamics, we introduce a generalized d'Alembert wave equation that captures the many-body damping and retardation inherent to driven quantum systems. These results establish current-current response functions as a platform to harness qualitatively new collective dynamics in correlated matter, opening new avenues for probing light-matter interactions beyond charge-density dynamics.
format Preprint
id arxiv_https___arxiv_org_abs_2504_00583
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Driving collective current excitations using light: The two-time $GW$ approach
Ong, Chin Shen
Golež, Denis
Rubio, Angel
Eriksson, Olle
Strand, Hugo U. R.
Materials Science
We identify a distinct transverse collective excitation, which we name the "curron", arising from current-current interactions in a driven quantum metal. Unlike plasmons, which involve longitudinal charge oscillations, currons are transverse current-density oscillations resulting from the interplay between the vector potential generated by the current and the external driving field. We demonstrate the emergence of this excitation in sodium metal by solving the Kadanoff-Baym equations on a complex time contour within the non-equilibrium two-time (TT) $GW$ formalism, marking, to our knowledge, the first TT-$GW$ calculation on a realistic material. We further show that two-time quantum memory effects leave measurable signatures: a pump-induced elevation in the baseline of the current-to-field response, potentially observable in polarization- and momentum-resolved conductivity experiments. By extracting effective resistive and memory coefficients from the TT-$GW$ dynamics, we introduce a generalized d'Alembert wave equation that captures the many-body damping and retardation inherent to driven quantum systems. These results establish current-current response functions as a platform to harness qualitatively new collective dynamics in correlated matter, opening new avenues for probing light-matter interactions beyond charge-density dynamics.
title Driving collective current excitations using light: The two-time $GW$ approach
topic Materials Science
url https://arxiv.org/abs/2504.00583