Fully-gapped superconductivity with rotational symmetry breaking in pressurized kagome metal CsV$_3$Sb$_5$

Fuente: arXiv
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Autores principales: Feng, X. Y., Zhao, Z., Luo, J., Zhou, Y. Z., Yang, J., Fang, A. F., Yang, H. T., Gao, H. -J., Zhou, R., Zheng, Guo-qing
Formato: Preprint
Publicado: 2025
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author Feng, X. Y.
Zhao, Z.
Luo, J.
Zhou, Y. Z.
Yang, J.
Fang, A. F.
Yang, H. T.
Gao, H. -J.
Zhou, R.
Zheng, Guo-qing
author_facet Feng, X. Y.
Zhao, Z.
Luo, J.
Zhou, Y. Z.
Yang, J.
Fang, A. F.
Yang, H. T.
Gao, H. -J.
Zhou, R.
Zheng, Guo-qing
contents The discovery of the kagome metal CsV$_3$Sb$_5$ has generated significant interest in its complex physical properties, particularly its superconducting behavior under different pressures, though its nature remains debated. Here, we performed low-temperature, high-pressure $^{121/123}$Sb nuclear quadrupole resonance (NQR) measurements to explore the superconducting pairing symmetry in CsV$_3$Sb$_5$. At ambient pressure, we found that the spin-lattice relaxation rate 1/$T_1$ exhibits a kink at $T \sim$ 0.4 $T_\textrm{c}$ within the superconducting state and follows a $T^3$ variation as temperature further decreases. This suggests the presence of two superconducting gaps with line nodes in the smaller one. As pressure increases beyond $P_{\rm c} \sim 1.85$ GPa, where the charge-density wave phase is completely suppressed, 1/$T_1$ shows no Hebel-Slichter peak just below $T_\textrm{c}$, and decreases rapidly, even faster than $T^5$, indicating that the gap is fully opened for pressures above $P_{\rm c}$. In this high pressure region, the angular dependence of the in-plane upper critical magnetic field $H_{\rm c2}$ breaks the $C_6$ rotational symmetry. We propose the $s+id$ pairing at $P > P_{\rm c}$ which explains both the 1/$T_1$ and $H_{\rm c2}$ behaviors. Our findings indicate that CsV$_3$Sb$_5$ is an unconventional superconductor and its superconducting state is even more exotic at high pressures.
format Preprint
id arxiv_https___arxiv_org_abs_2504_01763
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Fully-gapped superconductivity with rotational symmetry breaking in pressurized kagome metal CsV$_3$Sb$_5$
Feng, X. Y.
Zhao, Z.
Luo, J.
Zhou, Y. Z.
Yang, J.
Fang, A. F.
Yang, H. T.
Gao, H. -J.
Zhou, R.
Zheng, Guo-qing
Superconductivity
Strongly Correlated Electrons
The discovery of the kagome metal CsV$_3$Sb$_5$ has generated significant interest in its complex physical properties, particularly its superconducting behavior under different pressures, though its nature remains debated. Here, we performed low-temperature, high-pressure $^{121/123}$Sb nuclear quadrupole resonance (NQR) measurements to explore the superconducting pairing symmetry in CsV$_3$Sb$_5$. At ambient pressure, we found that the spin-lattice relaxation rate 1/$T_1$ exhibits a kink at $T \sim$ 0.4 $T_\textrm{c}$ within the superconducting state and follows a $T^3$ variation as temperature further decreases. This suggests the presence of two superconducting gaps with line nodes in the smaller one. As pressure increases beyond $P_{\rm c} \sim 1.85$ GPa, where the charge-density wave phase is completely suppressed, 1/$T_1$ shows no Hebel-Slichter peak just below $T_\textrm{c}$, and decreases rapidly, even faster than $T^5$, indicating that the gap is fully opened for pressures above $P_{\rm c}$. In this high pressure region, the angular dependence of the in-plane upper critical magnetic field $H_{\rm c2}$ breaks the $C_6$ rotational symmetry. We propose the $s+id$ pairing at $P > P_{\rm c}$ which explains both the 1/$T_1$ and $H_{\rm c2}$ behaviors. Our findings indicate that CsV$_3$Sb$_5$ is an unconventional superconductor and its superconducting state is even more exotic at high pressures.
title Fully-gapped superconductivity with rotational symmetry breaking in pressurized kagome metal CsV$_3$Sb$_5$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2504.01763