Hybrid d/p-wave altermagnetism in Ca$_{3}$Ru$_{2}$O$_{7}$ and strain-controlled spin splitting

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Hauptverfasser: León, Andrea, Autieri, Carmine, Brumme, Thomas, González, Jhon W.
Format: Preprint
Veröffentlicht: 2025
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author León, Andrea
Autieri, Carmine
Brumme, Thomas
González, Jhon W.
author_facet León, Andrea
Autieri, Carmine
Brumme, Thomas
González, Jhon W.
contents The interplay of strong electronic correlations, sizable octahedral distortions, and pronounced spin-orbit coupling (SOC) makes perovskite oxides promising candidates for realizing altermagnetic phases. We study altermagnetic phases in Ca$_3$Ru$_2$O$_7$, a non-centrosymmetric layered perovskite whose ground state is a Kramers-degenerate antiferromagnet. We show that an alternative Néel-type spin arrangement hosts a P-2 d-wave altermagnetic state with orbital selectivity similar to Ca$_2$RuO$_4$. Including SOC generates a symmetry-allowed p-wave component and yields a hybrid d/p-wave altermagnetic order. We further demonstrate that biaxial strain tunes both magnetic stability and band splitting: compressive strain beyond 2 % favors the altermagnetic phase over the antiferromagnetic ground state, while tensile strain increases altermagnetic splittings by up to 9 %. To quantify these trends, we define an altermagnetic figure of merit and trace its strain dependence to changes in electronic localization and octahedral geometry in this polar metal.
format Preprint
id arxiv_https___arxiv_org_abs_2504_04552
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Hybrid d/p-wave altermagnetism in Ca$_{3}$Ru$_{2}$O$_{7}$ and strain-controlled spin splitting
León, Andrea
Autieri, Carmine
Brumme, Thomas
González, Jhon W.
Materials Science
The interplay of strong electronic correlations, sizable octahedral distortions, and pronounced spin-orbit coupling (SOC) makes perovskite oxides promising candidates for realizing altermagnetic phases. We study altermagnetic phases in Ca$_3$Ru$_2$O$_7$, a non-centrosymmetric layered perovskite whose ground state is a Kramers-degenerate antiferromagnet. We show that an alternative Néel-type spin arrangement hosts a P-2 d-wave altermagnetic state with orbital selectivity similar to Ca$_2$RuO$_4$. Including SOC generates a symmetry-allowed p-wave component and yields a hybrid d/p-wave altermagnetic order. We further demonstrate that biaxial strain tunes both magnetic stability and band splitting: compressive strain beyond 2 % favors the altermagnetic phase over the antiferromagnetic ground state, while tensile strain increases altermagnetic splittings by up to 9 %. To quantify these trends, we define an altermagnetic figure of merit and trace its strain dependence to changes in electronic localization and octahedral geometry in this polar metal.
title Hybrid d/p-wave altermagnetism in Ca$_{3}$Ru$_{2}$O$_{7}$ and strain-controlled spin splitting
topic Materials Science
url https://arxiv.org/abs/2504.04552