High-efficiency broadband active metasurfaces via reversible metal electrodeposition

Fuente: arXiv
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Autori principali: Li, Qizhang, Kulkarni, Sachin Prashant, Sui, Chenxi, Chen, Ting-Hsuan, Yan, Gangbin, Wu, Ronghui, Chen, Wen, Hung, Pei-Jan, Wu, Xubing, Emersic, Tadej, Aydin, Koray, Hsu, Po-Chun
Natura: Preprint
Pubblicazione: 2025
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author Li, Qizhang
Kulkarni, Sachin Prashant
Sui, Chenxi
Chen, Ting-Hsuan
Yan, Gangbin
Wu, Ronghui
Chen, Wen
Hung, Pei-Jan
Wu, Xubing
Emersic, Tadej
Aydin, Koray
Hsu, Po-Chun
author_facet Li, Qizhang
Kulkarni, Sachin Prashant
Sui, Chenxi
Chen, Ting-Hsuan
Yan, Gangbin
Wu, Ronghui
Chen, Wen
Hung, Pei-Jan
Wu, Xubing
Emersic, Tadej
Aydin, Koray
Hsu, Po-Chun
contents Realizing active metasurfaces with substantial tunability is important for many applications but remains challenging due to difficulties in dynamically tuning light-matter interactions at subwavelength scales. Here, we introduce reversible metal electrodeposition as a versatile approach for enabling active metasurfaces with exceptional tunability across a broad bandwidth. As a proof of concept, we demonstrate a dynamic beam-steering device by performing reversible copper (Cu) electrodeposition on a reflective gradient metasurface composed of metal-insulator-metal resonators. By applying different voltages, the Cu atoms can be uniformly and reversibly electrodeposited and stripped around the resonators, effectively controlling the gap-surface plasmon resonances and steering the reflected light. This process experimentally achieved >90% diffraction efficiencies and >60% reflection efficiencies in both specular and anomalous modes, even after thousands of cycles. Moreover, these high efficiencies can be extended from the visible to the near- and mid-infrared regimes, demonstrating the broad versatility of this approach in enabling various active optical and thermal devices with different working wavelengths and bandwidths.
format Preprint
id arxiv_https___arxiv_org_abs_2504_05612
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle High-efficiency broadband active metasurfaces via reversible metal electrodeposition
Li, Qizhang
Kulkarni, Sachin Prashant
Sui, Chenxi
Chen, Ting-Hsuan
Yan, Gangbin
Wu, Ronghui
Chen, Wen
Hung, Pei-Jan
Wu, Xubing
Emersic, Tadej
Aydin, Koray
Hsu, Po-Chun
Optics
Materials Science
Applied Physics
Realizing active metasurfaces with substantial tunability is important for many applications but remains challenging due to difficulties in dynamically tuning light-matter interactions at subwavelength scales. Here, we introduce reversible metal electrodeposition as a versatile approach for enabling active metasurfaces with exceptional tunability across a broad bandwidth. As a proof of concept, we demonstrate a dynamic beam-steering device by performing reversible copper (Cu) electrodeposition on a reflective gradient metasurface composed of metal-insulator-metal resonators. By applying different voltages, the Cu atoms can be uniformly and reversibly electrodeposited and stripped around the resonators, effectively controlling the gap-surface plasmon resonances and steering the reflected light. This process experimentally achieved >90% diffraction efficiencies and >60% reflection efficiencies in both specular and anomalous modes, even after thousands of cycles. Moreover, these high efficiencies can be extended from the visible to the near- and mid-infrared regimes, demonstrating the broad versatility of this approach in enabling various active optical and thermal devices with different working wavelengths and bandwidths.
title High-efficiency broadband active metasurfaces via reversible metal electrodeposition
topic Optics
Materials Science
Applied Physics
url https://arxiv.org/abs/2504.05612