Layer-dependent field-free switching of Néel vector in a van der Waals antiferromagnet

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Main Authors: Guo, Haoran, Lin, Zhongchong, Lu, Jinhao, Yun, Chao, Han, Guanghui, Sun, Shoutong, Wu, Yu, Yang, Wenyun, Xiao, Dongdong, Zhu, Zhifeng, Peng, Licong, Ye, Yu, Hou, Yanglong, Yang, Jinbo, Luo, Zhaochu
Format: Preprint
Published: 2025
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author Guo, Haoran
Lin, Zhongchong
Lu, Jinhao
Yun, Chao
Han, Guanghui
Sun, Shoutong
Wu, Yu
Yang, Wenyun
Xiao, Dongdong
Zhu, Zhifeng
Peng, Licong
Ye, Yu
Hou, Yanglong
Yang, Jinbo
Luo, Zhaochu
author_facet Guo, Haoran
Lin, Zhongchong
Lu, Jinhao
Yun, Chao
Han, Guanghui
Sun, Shoutong
Wu, Yu
Yang, Wenyun
Xiao, Dongdong
Zhu, Zhifeng
Peng, Licong
Ye, Yu
Hou, Yanglong
Yang, Jinbo
Luo, Zhaochu
contents Two-dimensional antiferromagnets, combining the dual advantages of van der Waals (vdW) and antiferromagnetic materials, provide an unprecedented platform for exploring emergent spin-related phenomena. However, electrical manipulation of Néel vectors in vdW antiferromagnets - the cornerstone of antiferromagnetic spintronics - remains challenging. Here, we report layer-dependent electrical switching of the Néel vector in an A-type vdW antiferromagnet $(Fe,Co)_3$$GaTe_2$ (FCGT) with perpendicular magnetic anisotropy. The Néel vector of FCGT with odd-number vdW layers can be 180° reversed via spin-orbit torques. Furthermore, we achieve field-free switching in an all-vdW, all-antiferromagnet heterostructure of FCGT/CrSBr in which the noncollinear interfacial spin texture breaks the mirror symmetry. Our results establish layer-controlled spin symmetries and interfacial spin engineering as universal paradigms for manipulating antiferromagnetic order, paving the way for realising reliable and efficient vdW antiferromagnetic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2504_06764
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Layer-dependent field-free switching of Néel vector in a van der Waals antiferromagnet
Guo, Haoran
Lin, Zhongchong
Lu, Jinhao
Yun, Chao
Han, Guanghui
Sun, Shoutong
Wu, Yu
Yang, Wenyun
Xiao, Dongdong
Zhu, Zhifeng
Peng, Licong
Ye, Yu
Hou, Yanglong
Yang, Jinbo
Luo, Zhaochu
Mesoscale and Nanoscale Physics
Two-dimensional antiferromagnets, combining the dual advantages of van der Waals (vdW) and antiferromagnetic materials, provide an unprecedented platform for exploring emergent spin-related phenomena. However, electrical manipulation of Néel vectors in vdW antiferromagnets - the cornerstone of antiferromagnetic spintronics - remains challenging. Here, we report layer-dependent electrical switching of the Néel vector in an A-type vdW antiferromagnet $(Fe,Co)_3$$GaTe_2$ (FCGT) with perpendicular magnetic anisotropy. The Néel vector of FCGT with odd-number vdW layers can be 180° reversed via spin-orbit torques. Furthermore, we achieve field-free switching in an all-vdW, all-antiferromagnet heterostructure of FCGT/CrSBr in which the noncollinear interfacial spin texture breaks the mirror symmetry. Our results establish layer-controlled spin symmetries and interfacial spin engineering as universal paradigms for manipulating antiferromagnetic order, paving the way for realising reliable and efficient vdW antiferromagnetic devices.
title Layer-dependent field-free switching of Néel vector in a van der Waals antiferromagnet
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2504.06764