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Main Authors: Kim, Na Yeon, Zhong, Hanfeng, Zhang, Jianhua, O'Leary, Colum M., Liao, Yuxuan, Zou, Ji, Sha, Haozhi, Pham, Minh, Li, Weiyi, Yuan, Yakun, Park, Ji-Hoon, Kim, Dennis, Jiang, Huaidong, Kong, Jing, Chi, Miaofang, Miao, Jianwei
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2504.08228
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author Kim, Na Yeon
Zhong, Hanfeng
Zhang, Jianhua
O'Leary, Colum M.
Liao, Yuxuan
Zou, Ji
Sha, Haozhi
Pham, Minh
Li, Weiyi
Yuan, Yakun
Park, Ji-Hoon
Kim, Dennis
Jiang, Huaidong
Kong, Jing
Chi, Miaofang
Miao, Jianwei
author_facet Kim, Na Yeon
Zhong, Hanfeng
Zhang, Jianhua
O'Leary, Colum M.
Liao, Yuxuan
Zou, Ji
Sha, Haozhi
Pham, Minh
Li, Weiyi
Yuan, Yakun
Park, Ji-Hoon
Kim, Dennis
Jiang, Huaidong
Kong, Jing
Chi, Miaofang
Miao, Jianwei
contents Carbon is fundamental to science and technology due to its diverse bonding configurations, structural versatility, and essential role in defining the mechanical, chemical, electronic, and quantum properties of materials. However, direct three-dimensional (3D) imaging of individual carbon atoms remains a long-standing challenge. Here, we use twisted bilayer graphene (TBG) as a model system and demonstrate ptychographic atomic electron tomography (pAET) for determining the 3D atomic coordinates of individual carbon atoms with a precision of 0.11 angstrom. The resulting 3D atomic model uncovers chiral lattice distortions driven by van der Waals interactions that exhibit meron-like and skyrmion-like structural textures. These findings provide direct insight into the interplay between 3D chiral lattice deformation and electronic properties in moire-engineered carbon systems. Beyond TBG, pAET offers a versatile approach for 3D atomic-scale imaging of carbon-based and other light-element materials that are central to advances in physics, chemistry, materials science, and nanotechnology.
format Preprint
id arxiv_https___arxiv_org_abs_2504_08228
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Three-dimensional imaging of individual carbon atoms
Kim, Na Yeon
Zhong, Hanfeng
Zhang, Jianhua
O'Leary, Colum M.
Liao, Yuxuan
Zou, Ji
Sha, Haozhi
Pham, Minh
Li, Weiyi
Yuan, Yakun
Park, Ji-Hoon
Kim, Dennis
Jiang, Huaidong
Kong, Jing
Chi, Miaofang
Miao, Jianwei
Materials Science
Instrumentation and Detectors
Carbon is fundamental to science and technology due to its diverse bonding configurations, structural versatility, and essential role in defining the mechanical, chemical, electronic, and quantum properties of materials. However, direct three-dimensional (3D) imaging of individual carbon atoms remains a long-standing challenge. Here, we use twisted bilayer graphene (TBG) as a model system and demonstrate ptychographic atomic electron tomography (pAET) for determining the 3D atomic coordinates of individual carbon atoms with a precision of 0.11 angstrom. The resulting 3D atomic model uncovers chiral lattice distortions driven by van der Waals interactions that exhibit meron-like and skyrmion-like structural textures. These findings provide direct insight into the interplay between 3D chiral lattice deformation and electronic properties in moire-engineered carbon systems. Beyond TBG, pAET offers a versatile approach for 3D atomic-scale imaging of carbon-based and other light-element materials that are central to advances in physics, chemistry, materials science, and nanotechnology.
title Three-dimensional imaging of individual carbon atoms
topic Materials Science
Instrumentation and Detectors
url https://arxiv.org/abs/2504.08228