Active stabilization for ultralong acquisitions in an attosecond pump-probe beamline

Fuente: arXiv
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Autores principales: Csizmadia, Tamás, Oldal, Lénárd Gulyás, Gilicze, Barnabás, Kiss, Dániel Sándor, Bartyik, Tamás, Varjú, Katalin, Kahaly, Subhendu, Major, Balázs
Formato: Preprint
Publicado: 2025
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author Csizmadia, Tamás
Oldal, Lénárd Gulyás
Gilicze, Barnabás
Kiss, Dániel Sándor
Bartyik, Tamás
Varjú, Katalin
Kahaly, Subhendu
Major, Balázs
author_facet Csizmadia, Tamás
Oldal, Lénárd Gulyás
Gilicze, Barnabás
Kiss, Dániel Sándor
Bartyik, Tamás
Varjú, Katalin
Kahaly, Subhendu
Major, Balázs
contents Attosecond time-resolution experiments using noncollinear interferometers require precise and active control of the optical delay to prevent instabilities - including both slow drifts and rapid vibrations - that can obscure the time evolution of the physical system under investigation. In this work, we present the design and results of stability measurements for a double interferometer setup for extreme ultraviolet-infrared pump-probe spectroscopy. The attosecond pump-probe setup is driven by a high-average-power, high-repetition-rate laser system and offers sub-optical-cycle (+/-81 as) stability with a fast feedback rate over extended periods (up to several days). Due to the noncollinear arrangement, the setup enables independent control of both amplitude and phase in the two arms even across significantly different spectral regions. As a proof of concept, we demonstrate attosecond beating in angle-resolved photoemission during two-photon, two-color photoionization, highlighting the broad potential of the system for kinematically and dynamically complete studies of atomic-scale light-matter interactions.
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institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Active stabilization for ultralong acquisitions in an attosecond pump-probe beamline
Csizmadia, Tamás
Oldal, Lénárd Gulyás
Gilicze, Barnabás
Kiss, Dániel Sándor
Bartyik, Tamás
Varjú, Katalin
Kahaly, Subhendu
Major, Balázs
Optics
Atomic Physics
Attosecond time-resolution experiments using noncollinear interferometers require precise and active control of the optical delay to prevent instabilities - including both slow drifts and rapid vibrations - that can obscure the time evolution of the physical system under investigation. In this work, we present the design and results of stability measurements for a double interferometer setup for extreme ultraviolet-infrared pump-probe spectroscopy. The attosecond pump-probe setup is driven by a high-average-power, high-repetition-rate laser system and offers sub-optical-cycle (+/-81 as) stability with a fast feedback rate over extended periods (up to several days). Due to the noncollinear arrangement, the setup enables independent control of both amplitude and phase in the two arms even across significantly different spectral regions. As a proof of concept, we demonstrate attosecond beating in angle-resolved photoemission during two-photon, two-color photoionization, highlighting the broad potential of the system for kinematically and dynamically complete studies of atomic-scale light-matter interactions.
title Active stabilization for ultralong acquisitions in an attosecond pump-probe beamline
topic Optics
Atomic Physics
url https://arxiv.org/abs/2504.08448