Long-range magnetic interactions in Nd$_2$PdSi$_3$ and the formation of skyrmion phases in centrosymmetric metals

Fuente: arXiv
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Autores principales: Peçanha-Antonio, Viviane, Shan, Zhaoyang, Smidman, Michael, Bouaziz, Juba, Ouladdiaf, Bachir, Kibalin, Iurii, Lemee, Marie Helene, Balz, Christian, Lass, Jakob, Mayoh, Daniel A., Balakrishnan, Geetha, Staunton, Julie B., Adroja, Davashibhai, Boothroyd, Andrew T.
Formato: Preprint
Publicado: 2025
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author Peçanha-Antonio, Viviane
Shan, Zhaoyang
Smidman, Michael
Bouaziz, Juba
Ouladdiaf, Bachir
Kibalin, Iurii
Lemee, Marie Helene
Balz, Christian
Lass, Jakob
Mayoh, Daniel A.
Balakrishnan, Geetha
Staunton, Julie B.
Adroja, Davashibhai
Boothroyd, Andrew T.
author_facet Peçanha-Antonio, Viviane
Shan, Zhaoyang
Smidman, Michael
Bouaziz, Juba
Ouladdiaf, Bachir
Kibalin, Iurii
Lemee, Marie Helene
Balz, Christian
Lass, Jakob
Mayoh, Daniel A.
Balakrishnan, Geetha
Staunton, Julie B.
Adroja, Davashibhai
Boothroyd, Andrew T.
contents We present an extensive X-ray and neutron scattering study of the structure and magnetic excitations of Nd$_2$PdSi$_3$, a sister compound of Gd$_2$PdSi$_3$ which was recently found to host a skyrmion lattice phase despite its centrosymmetric crystal structure. Dispersive magnetic excitations were measured throughout the Brillouin zone and modeled to determine the magnetic interactions between Nd ions. Our analysis reveals that the magnetic interactions in this system extend over large distances and are significantly affected by a crystallographic superstructure formed by ordering of the Pd and Si atoms. The results suggest that the mechanism for the skyrmion phase formation in this family of materials, specifically Gd$_2$PdSi$_3$, is through the long-range RKKY interactions rather than short-range triangular-lattice frustration.
format Preprint
id arxiv_https___arxiv_org_abs_2504_10075
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Long-range magnetic interactions in Nd$_2$PdSi$_3$ and the formation of skyrmion phases in centrosymmetric metals
Peçanha-Antonio, Viviane
Shan, Zhaoyang
Smidman, Michael
Bouaziz, Juba
Ouladdiaf, Bachir
Kibalin, Iurii
Lemee, Marie Helene
Balz, Christian
Lass, Jakob
Mayoh, Daniel A.
Balakrishnan, Geetha
Staunton, Julie B.
Adroja, Davashibhai
Boothroyd, Andrew T.
Strongly Correlated Electrons
Other Condensed Matter
We present an extensive X-ray and neutron scattering study of the structure and magnetic excitations of Nd$_2$PdSi$_3$, a sister compound of Gd$_2$PdSi$_3$ which was recently found to host a skyrmion lattice phase despite its centrosymmetric crystal structure. Dispersive magnetic excitations were measured throughout the Brillouin zone and modeled to determine the magnetic interactions between Nd ions. Our analysis reveals that the magnetic interactions in this system extend over large distances and are significantly affected by a crystallographic superstructure formed by ordering of the Pd and Si atoms. The results suggest that the mechanism for the skyrmion phase formation in this family of materials, specifically Gd$_2$PdSi$_3$, is through the long-range RKKY interactions rather than short-range triangular-lattice frustration.
title Long-range magnetic interactions in Nd$_2$PdSi$_3$ and the formation of skyrmion phases in centrosymmetric metals
topic Strongly Correlated Electrons
Other Condensed Matter
url https://arxiv.org/abs/2504.10075