Isomeric yield ratios and mass spectrometry of Y and Nb isotopes in the neutron-rich N=60 region: the unusual case of $^{98}$Y

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Hauptverfasser: Cannarozzo, Simone, Pomp, Stephan, Kankainen, Anu, Moore, Iain, Stryjczyk, Marek, Al-Adili, Ali, Solders, Andreas, Virtanen, Ville, Eronen, Tommi, Gao, Zhihao, Ge, Zhuang, Jaries, Arthur, Lantz, Mattias, Mougeot, Maxime, Penttilä, Heikki, Raggio, Andrea, Ruotsalainen, Jouni
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Veröffentlicht: 2025
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author Cannarozzo, Simone
Pomp, Stephan
Kankainen, Anu
Moore, Iain
Stryjczyk, Marek
Al-Adili, Ali
Solders, Andreas
Virtanen, Ville
Eronen, Tommi
Gao, Zhihao
Ge, Zhuang
Jaries, Arthur
Lantz, Mattias
Mougeot, Maxime
Penttilä, Heikki
Raggio, Andrea
Ruotsalainen, Jouni
author_facet Cannarozzo, Simone
Pomp, Stephan
Kankainen, Anu
Moore, Iain
Stryjczyk, Marek
Al-Adili, Ali
Solders, Andreas
Virtanen, Ville
Eronen, Tommi
Gao, Zhihao
Ge, Zhuang
Jaries, Arthur
Lantz, Mattias
Mougeot, Maxime
Penttilä, Heikki
Raggio, Andrea
Ruotsalainen, Jouni
contents The isomeric yield ratio (IYR) of fission products is an observable that carries relevant information about the fragments emerging from the scission of a fissioning nucleus. We report on IYR of $^{96,98,100}$Y and $^{100,102}$Nb, together with the previously reported values for $^{97}$Y and $^{99}$Nb, produced in the 28 MeV $α$-induced fission of $^{232}$Th at the Ion Guide Isotope Separation On-Line (IGISOL) facility of the University of Jyv{ä}skyl{ä}. We measured the IYR using two different techniques, the phase-imaging ion-cyclotron-resonance (PI-ICR) and the multiple-reflection time-of-flight mass spectrometry (MR-TOF-MS) methods. Moreover, we measured the masses of the long-lived states in $^{98,100}$Y and $^{100,102}$Nb populated via in-trap $β$-decay of their precursors. Since the $β$-decay selectively populates states with a favourable spin-parity, we could identify the measured state and show that the ground state is the low-spin state in the cases of $^{98}$Y and $^{100}$Nb, while it is the high-spin state in the cases of $^{100}$Y and $^{102}$Nb. This measurement confirms the spin-parity assignments of all the nuclei as they are reported in the NUBASE2020 evaluations, disagreeing with the assignment for $^{100}$Y reported in the ENSDF evaluation. Making also use of previously reported data, we observe an anomalously low IYR for the $N=59$ isotope $^{98}$Y as compared to other yttrium or neighboring niobium isotopes. This behavior is very rare across the nuclear chart and is posited to be connected to the characteristic shape coexistence of $^{98}$Y, and to the change in the charge radii of the ground and excited states in the $N=58-60$ region.
format Preprint
id arxiv_https___arxiv_org_abs_2504_11274
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Isomeric yield ratios and mass spectrometry of Y and Nb isotopes in the neutron-rich N=60 region: the unusual case of $^{98}$Y
Cannarozzo, Simone
Pomp, Stephan
Kankainen, Anu
Moore, Iain
Stryjczyk, Marek
Al-Adili, Ali
Solders, Andreas
Virtanen, Ville
Eronen, Tommi
Gao, Zhihao
Ge, Zhuang
Jaries, Arthur
Lantz, Mattias
Mougeot, Maxime
Penttilä, Heikki
Raggio, Andrea
Ruotsalainen, Jouni
Nuclear Experiment
The isomeric yield ratio (IYR) of fission products is an observable that carries relevant information about the fragments emerging from the scission of a fissioning nucleus. We report on IYR of $^{96,98,100}$Y and $^{100,102}$Nb, together with the previously reported values for $^{97}$Y and $^{99}$Nb, produced in the 28 MeV $α$-induced fission of $^{232}$Th at the Ion Guide Isotope Separation On-Line (IGISOL) facility of the University of Jyv{ä}skyl{ä}. We measured the IYR using two different techniques, the phase-imaging ion-cyclotron-resonance (PI-ICR) and the multiple-reflection time-of-flight mass spectrometry (MR-TOF-MS) methods. Moreover, we measured the masses of the long-lived states in $^{98,100}$Y and $^{100,102}$Nb populated via in-trap $β$-decay of their precursors. Since the $β$-decay selectively populates states with a favourable spin-parity, we could identify the measured state and show that the ground state is the low-spin state in the cases of $^{98}$Y and $^{100}$Nb, while it is the high-spin state in the cases of $^{100}$Y and $^{102}$Nb. This measurement confirms the spin-parity assignments of all the nuclei as they are reported in the NUBASE2020 evaluations, disagreeing with the assignment for $^{100}$Y reported in the ENSDF evaluation. Making also use of previously reported data, we observe an anomalously low IYR for the $N=59$ isotope $^{98}$Y as compared to other yttrium or neighboring niobium isotopes. This behavior is very rare across the nuclear chart and is posited to be connected to the characteristic shape coexistence of $^{98}$Y, and to the change in the charge radii of the ground and excited states in the $N=58-60$ region.
title Isomeric yield ratios and mass spectrometry of Y and Nb isotopes in the neutron-rich N=60 region: the unusual case of $^{98}$Y
topic Nuclear Experiment
url https://arxiv.org/abs/2504.11274