Probing Quantum Anomalous Hall States in Twisted Bilayer WSe2 via Attractive Polaron Spectroscopy

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Hauptverfasser: Gao, Beini, Ghafariasl, Mahdi, Mehrabad, Mahmoud Jalali, Huang, Tsung-Sheng, Zhang, Lifu, Session, Deric, Upadhyay, Pranshoo, Ma, Rundong, Alshalan, Ghadah, Forero, Daniel Gustavo Suárez, Sarkar, Supratik, Park, Suji, Jang, Houk, Watanabe, Kenji, Taniguchi, Takashi, Xie, Ming, Zhou, You, Hafezi, Mohammad
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Veröffentlicht: 2025
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author Gao, Beini
Ghafariasl, Mahdi
Mehrabad, Mahmoud Jalali
Huang, Tsung-Sheng
Zhang, Lifu
Session, Deric
Upadhyay, Pranshoo
Ma, Rundong
Alshalan, Ghadah
Forero, Daniel Gustavo Suárez
Sarkar, Supratik
Park, Suji
Jang, Houk
Watanabe, Kenji
Taniguchi, Takashi
Xie, Ming
Zhou, You
Hafezi, Mohammad
author_facet Gao, Beini
Ghafariasl, Mahdi
Mehrabad, Mahmoud Jalali
Huang, Tsung-Sheng
Zhang, Lifu
Session, Deric
Upadhyay, Pranshoo
Ma, Rundong
Alshalan, Ghadah
Forero, Daniel Gustavo Suárez
Sarkar, Supratik
Park, Suji
Jang, Houk
Watanabe, Kenji
Taniguchi, Takashi
Xie, Ming
Zhou, You
Hafezi, Mohammad
contents Moiré superlattices in semiconductors exhibit a rich variety of interaction-induced topological states, including quantum anomalous Hall (QAH) effects. A recent study hinted that twisted WSe2 homobilayer (tWSe2) could host a QAH state but lacked direct evidence of ferromagnetism, a key hallmark of this phase. Here, we report the first direct evidence of QAH states in tWSe2 with spontaneous ferromagnetism. Specifically, we employ polarization-resolved attractive polaron spectroscopy on a dual-gated, 2 degree tWSe2 and observe direct signatures of spontaneous time-reversal symmetry breaking at hole filling ν= 1. Together with a Chern number measurement via Streda formula analysis, we identify this magnetized state as a topological state, characterized by C = 1. Furthermore, we demonstrate that these topological and magnetic properties are tunable via a finite displacement field, between a QAH ferromagnetic state and an antiferromagnetic state. Our findings position tWSe2 as a highly versatile, stable, and optically addressable platform for investigating topological order and strong correlations in two-dimensional landscapes.
format Preprint
id arxiv_https___arxiv_org_abs_2504_11530
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Probing Quantum Anomalous Hall States in Twisted Bilayer WSe2 via Attractive Polaron Spectroscopy
Gao, Beini
Ghafariasl, Mahdi
Mehrabad, Mahmoud Jalali
Huang, Tsung-Sheng
Zhang, Lifu
Session, Deric
Upadhyay, Pranshoo
Ma, Rundong
Alshalan, Ghadah
Forero, Daniel Gustavo Suárez
Sarkar, Supratik
Park, Suji
Jang, Houk
Watanabe, Kenji
Taniguchi, Takashi
Xie, Ming
Zhou, You
Hafezi, Mohammad
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
Quantum Physics
Moiré superlattices in semiconductors exhibit a rich variety of interaction-induced topological states, including quantum anomalous Hall (QAH) effects. A recent study hinted that twisted WSe2 homobilayer (tWSe2) could host a QAH state but lacked direct evidence of ferromagnetism, a key hallmark of this phase. Here, we report the first direct evidence of QAH states in tWSe2 with spontaneous ferromagnetism. Specifically, we employ polarization-resolved attractive polaron spectroscopy on a dual-gated, 2 degree tWSe2 and observe direct signatures of spontaneous time-reversal symmetry breaking at hole filling ν= 1. Together with a Chern number measurement via Streda formula analysis, we identify this magnetized state as a topological state, characterized by C = 1. Furthermore, we demonstrate that these topological and magnetic properties are tunable via a finite displacement field, between a QAH ferromagnetic state and an antiferromagnetic state. Our findings position tWSe2 as a highly versatile, stable, and optically addressable platform for investigating topological order and strong correlations in two-dimensional landscapes.
title Probing Quantum Anomalous Hall States in Twisted Bilayer WSe2 via Attractive Polaron Spectroscopy
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
Quantum Physics
url https://arxiv.org/abs/2504.11530