X-ray scattering investigation of hydride surface segregation in epitaxial Nb films

Fuente: arXiv
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Bibliographic Details
Main Authors: Garcia-Wetten, David A., Ryan, Philip J., Kim, Jong Woo, Goronzy, Dominic P, Reinertsen, Roger J., Hersam, Mark C., Bedzyk, Michael J.
Format: Preprint
Published: 2025
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_version_ 1866910912497057792
author Garcia-Wetten, David A.
Ryan, Philip J.
Kim, Jong Woo
Goronzy, Dominic P
Reinertsen, Roger J.
Hersam, Mark C.
Bedzyk, Michael J.
author_facet Garcia-Wetten, David A.
Ryan, Philip J.
Kim, Jong Woo
Goronzy, Dominic P
Reinertsen, Roger J.
Hersam, Mark C.
Bedzyk, Michael J.
contents Hydride precipitation in niobium-based, superconducting circuits is a damaging side-effect of hydrofluoric acid treatments used to clean and thin the Nb surface oxides and Si oxides. The precipitate microstructure is difficult to probe because of the high hydrogen mobility in the niobium matrix. In particular, destructive techniques used to prepare samples for elemental depth profiling can change the hydride structure. Here, we use X-ray surface scattering to non-destructively probe the depth distribution of precipitates in hydrided, epitaxial, niobium thin films. We find that the niobium hydride is confined within the top ten nm of the surface.
format Preprint
id arxiv_https___arxiv_org_abs_2504_11573
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle X-ray scattering investigation of hydride surface segregation in epitaxial Nb films
Garcia-Wetten, David A.
Ryan, Philip J.
Kim, Jong Woo
Goronzy, Dominic P
Reinertsen, Roger J.
Hersam, Mark C.
Bedzyk, Michael J.
Materials Science
Hydride precipitation in niobium-based, superconducting circuits is a damaging side-effect of hydrofluoric acid treatments used to clean and thin the Nb surface oxides and Si oxides. The precipitate microstructure is difficult to probe because of the high hydrogen mobility in the niobium matrix. In particular, destructive techniques used to prepare samples for elemental depth profiling can change the hydride structure. Here, we use X-ray surface scattering to non-destructively probe the depth distribution of precipitates in hydrided, epitaxial, niobium thin films. We find that the niobium hydride is confined within the top ten nm of the surface.
title X-ray scattering investigation of hydride surface segregation in epitaxial Nb films
topic Materials Science
url https://arxiv.org/abs/2504.11573