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Auteurs principaux: Shi, Yihan, Pan, Qingrui, Li, Jitao, Shi, Xiaoze, Wang, Youchang, Xiao, Peng
Format: Preprint
Publié: 2025
Sujets:
Accès en ligne:https://arxiv.org/abs/2504.11861
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author Shi, Yihan
Pan, Qingrui
Li, Jitao
Shi, Xiaoze
Wang, Youchang
Xiao, Peng
author_facet Shi, Yihan
Pan, Qingrui
Li, Jitao
Shi, Xiaoze
Wang, Youchang
Xiao, Peng
contents This work presents a comprehensive study on the aging behavior of 18650-type lithium-ion batteries, focusing on the uneven intercalation of lithium ions during fast charging processes. It introduces a novel approach using color visual recognition technology to analyze color changes in the graphite anode, indicative of lithiation levels. The study employs X-ray diffraction (XRD) and Distribution of Relaxation Time (DRT) techniques to validate and analyze the observations. The study emphasizes the significance of electrode impedance, the positioning of battery tabs, and electrolyte distribution in influencing the aging dynamics of lithium-ion batteries. Furthermore, the paper presents an innovative impedance Transport-Line Model, specifically developed to capture the evolution of polarization impedance over time. This model offers a deeper understanding of the internal mechanisms driving battery aging, providing valuable insights for the design and optimization of lithium-ion batteries. The research represents a significant contribution to the field, shedding light on the complex aging processes in lithium-ion batteries, particularly under the conditions of fast charging. This could lead to improved battery performance, longevity, and safety, which are critical for the wide range of applications that depend on these energy storage systems.
format Preprint
id arxiv_https___arxiv_org_abs_2504_11861
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Visualization Analysis and Impedance Analysis for the Aging Behavior Assessment of 18650 Cells
Shi, Yihan
Pan, Qingrui
Li, Jitao
Shi, Xiaoze
Wang, Youchang
Xiao, Peng
Materials Science
Applied Physics
This work presents a comprehensive study on the aging behavior of 18650-type lithium-ion batteries, focusing on the uneven intercalation of lithium ions during fast charging processes. It introduces a novel approach using color visual recognition technology to analyze color changes in the graphite anode, indicative of lithiation levels. The study employs X-ray diffraction (XRD) and Distribution of Relaxation Time (DRT) techniques to validate and analyze the observations. The study emphasizes the significance of electrode impedance, the positioning of battery tabs, and electrolyte distribution in influencing the aging dynamics of lithium-ion batteries. Furthermore, the paper presents an innovative impedance Transport-Line Model, specifically developed to capture the evolution of polarization impedance over time. This model offers a deeper understanding of the internal mechanisms driving battery aging, providing valuable insights for the design and optimization of lithium-ion batteries. The research represents a significant contribution to the field, shedding light on the complex aging processes in lithium-ion batteries, particularly under the conditions of fast charging. This could lead to improved battery performance, longevity, and safety, which are critical for the wide range of applications that depend on these energy storage systems.
title Visualization Analysis and Impedance Analysis for the Aging Behavior Assessment of 18650 Cells
topic Materials Science
Applied Physics
url https://arxiv.org/abs/2504.11861