Strong-coupling study of the pairing mechanism in pressurized La$_3$Ni$_2$O$_7$

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Hauptverfasser: Ji, Jia-Heng, Lu, Chen, Shao, Zhi-Yan, Pan, Zhiming, Yang, Fan, Wu, Congjun
Format: Preprint
Veröffentlicht: 2025
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author Ji, Jia-Heng
Lu, Chen
Shao, Zhi-Yan
Pan, Zhiming
Yang, Fan
Wu, Congjun
author_facet Ji, Jia-Heng
Lu, Chen
Shao, Zhi-Yan
Pan, Zhiming
Yang, Fan
Wu, Congjun
contents Recently, the bilayer perovskite nickelate La$_3$Ni$_2$O$_7$ has been reported to exhibit high-temperature superconductivity near $80$ K under a moderate pressure of about $14$GPa. To investigate the underlying pairing mechanism and symmetry in this complex system, we propose and analyze a mixed spin-$1$ and spin-$\frac{1}{2}$ bilayer $t$-$J$ model in the strong coupling regime. This model explicitly incorporates the crucial role of strong Hund's coupling, which favors the formation of local spin-triplet states from the two onsite $E_g$ orbital electrons at half-filling. We further investigate the model using both slave-particle mean-field theory and the density matrix renormalization group method. Our simulation results reveal that the dominate pairing channel is the interlayer one in the $3d_{x^2-y^2}$ orbital. The Hund's coupling is shown to enhance superconductivity within a reasonable physical range. Moreover, electron doping strengthens superconductivity by increasing carrier density; in contrast, hole doping weakens superconductivity. These findings offer critical insights into the unconventional superconductivity of pressurized La$_3$Ni$_2$O$_7$ and underline the important role of orbital-selective behavior and Hund's rule.
format Preprint
id arxiv_https___arxiv_org_abs_2504_12127
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Strong-coupling study of the pairing mechanism in pressurized La$_3$Ni$_2$O$_7$
Ji, Jia-Heng
Lu, Chen
Shao, Zhi-Yan
Pan, Zhiming
Yang, Fan
Wu, Congjun
Superconductivity
Strongly Correlated Electrons
Recently, the bilayer perovskite nickelate La$_3$Ni$_2$O$_7$ has been reported to exhibit high-temperature superconductivity near $80$ K under a moderate pressure of about $14$GPa. To investigate the underlying pairing mechanism and symmetry in this complex system, we propose and analyze a mixed spin-$1$ and spin-$\frac{1}{2}$ bilayer $t$-$J$ model in the strong coupling regime. This model explicitly incorporates the crucial role of strong Hund's coupling, which favors the formation of local spin-triplet states from the two onsite $E_g$ orbital electrons at half-filling. We further investigate the model using both slave-particle mean-field theory and the density matrix renormalization group method. Our simulation results reveal that the dominate pairing channel is the interlayer one in the $3d_{x^2-y^2}$ orbital. The Hund's coupling is shown to enhance superconductivity within a reasonable physical range. Moreover, electron doping strengthens superconductivity by increasing carrier density; in contrast, hole doping weakens superconductivity. These findings offer critical insights into the unconventional superconductivity of pressurized La$_3$Ni$_2$O$_7$ and underline the important role of orbital-selective behavior and Hund's rule.
title Strong-coupling study of the pairing mechanism in pressurized La$_3$Ni$_2$O$_7$
topic Superconductivity
Strongly Correlated Electrons
url https://arxiv.org/abs/2504.12127