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Main Authors: Chen, Yucong, Schertenleib, Till, Yang, Andrew, Schouwink, Pascal, Queen, Wendy L., Billinge, Simon J. L.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2504.12499
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author Chen, Yucong
Schertenleib, Till
Yang, Andrew
Schouwink, Pascal
Queen, Wendy L.
Billinge, Simon J. L.
author_facet Chen, Yucong
Schertenleib, Till
Yang, Andrew
Schouwink, Pascal
Queen, Wendy L.
Billinge, Simon J. L.
contents This paper explores the development and testing of a simple absorption correction model for processing x-ray powder diffraction data from Debye-Scherrer geometry laboratory x-ray experiments. This may be used as a pre-processing step before using PDFgetX3 to obtain reliable pair distribution functions (PDFs). The correction was found to depend only on muD, the product of the x-ray attenuation coefficient and capillary diameter. Various experimental and theoretical methods for estimating muD were explored, and the most appropriate muD values for correction were identified for different capillary diameters and x-ray beam sizes. We identify operational ranges of muD where reasonable signal to noise is possible after correction. A user-friendly software package, diffpy.labpdfproc, is presented that can help estimate muD and perform absorption corrections, with a rapid calculation for efficient processing.
format Preprint
id arxiv_https___arxiv_org_abs_2504_12499
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle An Absorption Correction for Reliable Pair-Distribution Functions from Low Energy X-ray Sources
Chen, Yucong
Schertenleib, Till
Yang, Andrew
Schouwink, Pascal
Queen, Wendy L.
Billinge, Simon J. L.
Materials Science
This paper explores the development and testing of a simple absorption correction model for processing x-ray powder diffraction data from Debye-Scherrer geometry laboratory x-ray experiments. This may be used as a pre-processing step before using PDFgetX3 to obtain reliable pair distribution functions (PDFs). The correction was found to depend only on muD, the product of the x-ray attenuation coefficient and capillary diameter. Various experimental and theoretical methods for estimating muD were explored, and the most appropriate muD values for correction were identified for different capillary diameters and x-ray beam sizes. We identify operational ranges of muD where reasonable signal to noise is possible after correction. A user-friendly software package, diffpy.labpdfproc, is presented that can help estimate muD and perform absorption corrections, with a rapid calculation for efficient processing.
title An Absorption Correction for Reliable Pair-Distribution Functions from Low Energy X-ray Sources
topic Materials Science
url https://arxiv.org/abs/2504.12499