Broadband Fourier transform spectroscopy of quantum emitters photoluminescence with sub-nanosecond temporal resolution

Fuente: arXiv
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Autori principali: Belgacem, Issam, Cilibrizzi, Pasquale, Arshad, Muhammad Junaid, White, Daniel, Kroj, Malte, Bekker, Christiaan, Mazzera, Margherita, Gerardot, Brian D., Frangeskou, Angelo C., Morley, Gavin W., Son, Nguyen Tien, Ul-Hassan, Jawad, Ohshima, Takeshi, Abe, Hiroshi, Vinco, Lorenzo, Polli, Dario, Cerullo, Giulio, Bonato, Cristian
Natura: Preprint
Pubblicazione: 2025
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author Belgacem, Issam
Cilibrizzi, Pasquale
Arshad, Muhammad Junaid
White, Daniel
Kroj, Malte
Bekker, Christiaan
Mazzera, Margherita
Gerardot, Brian D.
Frangeskou, Angelo C.
Morley, Gavin W.
Son, Nguyen Tien
Ul-Hassan, Jawad
Ohshima, Takeshi
Abe, Hiroshi
Vinco, Lorenzo
Polli, Dario
Cerullo, Giulio
Bonato, Cristian
author_facet Belgacem, Issam
Cilibrizzi, Pasquale
Arshad, Muhammad Junaid
White, Daniel
Kroj, Malte
Bekker, Christiaan
Mazzera, Margherita
Gerardot, Brian D.
Frangeskou, Angelo C.
Morley, Gavin W.
Son, Nguyen Tien
Ul-Hassan, Jawad
Ohshima, Takeshi
Abe, Hiroshi
Vinco, Lorenzo
Polli, Dario
Cerullo, Giulio
Bonato, Cristian
contents The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain Fourier transform spectroscopy, based on a compact and stable birefringent interferometer coupled to low-dark-count superconducting single-photon detectors, to the study of quantum emitters. We experimentally demonstrate that the system enables spectroscopy of quantum emitters over a broad wavelength interval from the near-infrared to the telecom range, where grating-based spectrometers coupled to InGaAs cameras are typically noisy and inefficient. We further show that the high temporal resolution of single-photon detectors, which can be on the order of tens of picoseconds, enables the monitoring of spin-dependent spectral changes on sub-nanosecond timescales.
format Preprint
id arxiv_https___arxiv_org_abs_2504_15258
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Broadband Fourier transform spectroscopy of quantum emitters photoluminescence with sub-nanosecond temporal resolution
Belgacem, Issam
Cilibrizzi, Pasquale
Arshad, Muhammad Junaid
White, Daniel
Kroj, Malte
Bekker, Christiaan
Mazzera, Margherita
Gerardot, Brian D.
Frangeskou, Angelo C.
Morley, Gavin W.
Son, Nguyen Tien
Ul-Hassan, Jawad
Ohshima, Takeshi
Abe, Hiroshi
Vinco, Lorenzo
Polli, Dario
Cerullo, Giulio
Bonato, Cristian
Quantum Physics
Mesoscale and Nanoscale Physics
Chemical Physics
Optics
The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain Fourier transform spectroscopy, based on a compact and stable birefringent interferometer coupled to low-dark-count superconducting single-photon detectors, to the study of quantum emitters. We experimentally demonstrate that the system enables spectroscopy of quantum emitters over a broad wavelength interval from the near-infrared to the telecom range, where grating-based spectrometers coupled to InGaAs cameras are typically noisy and inefficient. We further show that the high temporal resolution of single-photon detectors, which can be on the order of tens of picoseconds, enables the monitoring of spin-dependent spectral changes on sub-nanosecond timescales.
title Broadband Fourier transform spectroscopy of quantum emitters photoluminescence with sub-nanosecond temporal resolution
topic Quantum Physics
Mesoscale and Nanoscale Physics
Chemical Physics
Optics
url https://arxiv.org/abs/2504.15258