Two-step laser resonant ionization spectroscopy of chromium

Fuente: arXiv
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Main Authors: Schulz, Romina, Li, Ruohong, Wessolek, Julius, Mostamand, Maryam, Kunz, Peter, Lassen, Jens
Format: Preprint
Published: 2025
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_version_ 1866916702432788480
author Schulz, Romina
Li, Ruohong
Wessolek, Julius
Mostamand, Maryam
Kunz, Peter
Lassen, Jens
author_facet Schulz, Romina
Li, Ruohong
Wessolek, Julius
Mostamand, Maryam
Kunz, Peter
Lassen, Jens
contents At TRIUMF's off-line laser ion source test stand, stepwise resonant laser ionization spectroscopy of chromium (Cr) was carried out, to find an efficient ionization scheme suitable for titanium sapphire (Ti:Sa) laser systems. With three different first-excitation transitions, 357.971 nm, 359.451 nm, and 360.636 nm, automated continuous laser-frequency scans using a frequency-doubled, grating-tuned Ti:Sa laser were performed. Rydberg series as well as autoionizing(AI) states were observed. From these results, the ionization potential (IP) of Cr was determined as 54575.49(2)$_\text{stat}$(2)$_\text{sys}$ cm$^{-1}$, which is one order of magnitude more precise than the previously reported 54575.6(3) cm$^{-1}$ in NIST database. The ionization scheme using the observed AI resonance, with 357.971 nm as the first step and 373.935 nm as the second step was subsequently deployed to the online delivery of radioactive Cr isotope beams for precision mass measurements. The online yields of $^{50-59}$Cr have been measured at TRIUMF-ISAC.
format Preprint
id arxiv_https___arxiv_org_abs_2504_16067
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Two-step laser resonant ionization spectroscopy of chromium
Schulz, Romina
Li, Ruohong
Wessolek, Julius
Mostamand, Maryam
Kunz, Peter
Lassen, Jens
Atomic Physics
Accelerator Physics
Applied Physics
At TRIUMF's off-line laser ion source test stand, stepwise resonant laser ionization spectroscopy of chromium (Cr) was carried out, to find an efficient ionization scheme suitable for titanium sapphire (Ti:Sa) laser systems. With three different first-excitation transitions, 357.971 nm, 359.451 nm, and 360.636 nm, automated continuous laser-frequency scans using a frequency-doubled, grating-tuned Ti:Sa laser were performed. Rydberg series as well as autoionizing(AI) states were observed. From these results, the ionization potential (IP) of Cr was determined as 54575.49(2)$_\text{stat}$(2)$_\text{sys}$ cm$^{-1}$, which is one order of magnitude more precise than the previously reported 54575.6(3) cm$^{-1}$ in NIST database. The ionization scheme using the observed AI resonance, with 357.971 nm as the first step and 373.935 nm as the second step was subsequently deployed to the online delivery of radioactive Cr isotope beams for precision mass measurements. The online yields of $^{50-59}$Cr have been measured at TRIUMF-ISAC.
title Two-step laser resonant ionization spectroscopy of chromium
topic Atomic Physics
Accelerator Physics
Applied Physics
url https://arxiv.org/abs/2504.16067